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Experimental investigations and modelling of the ball motion in planetary ball mills
S. Rosenkranz , S. Breitung-Faes, A. Kwade
Institute for Particle Technology, TU Braunschweig, Braunschweig, Volkmaroder Strasse 5, 38104 Braunschweig, Germany
a r t i c l e
i n f o
Article history:
Received 1 November 2010
Received in revised form 26 April 2011
Accepted 21 May 2011
Available online 31 May 2011
Keywords:
Planetary ball mill
Ball motion
Discrete Element Method
Modelling
Stress energy
a b s t r a c t
Planetary ball mills feature attractive properties, like the possibility of dry or wet operation, straightforward
handling, cleanability and moderate costs. Consequently they are very well suited for lab scale process
development in diverse industries, including pharmaceuticals and new materials. A number of questions still
remain unanswered regarding this mill type. These include the stress conditions as well as transfer of the
grinding results to other types of mills with free moving balls, such as stirred media mills, which can be built in
large scales and operated continuously.
In order to measure the ball motion and, thus, the stress conditions, a planetary ball mill was equipped with a
high speed video camera, so that the grinding ball motion during the comminution process can be recorded
and analysed. The inuence of important process parameters on the ball motion pattern was assessed in this
study, namely speed ratio, ball lling ratio and friction conditions, the latter by applying different mill feeds.
The experimental results show considerable inuences of the ball lling ratio and friction conditions. The
measured ball motion patterns differ signicantly from ball trajectories which were calculated using kinetic
equations proposed in older publications.
In addition to the measurements the ball motion was simulated using a three dimensional Discrete Element
Model (DEM). An attempt was made to account for mill feed via altered friction coefcients. Correlations of
the DEM results and experimental ndings at different operating conditions show a good agreement. Based on
simulation data the frequency distribution of the stress energies in the mill could be calculated and compared
for different operating conditions.
2011 Elsevier B.V. All rights reserved.
1. Introduction
Due to their high energy density planetary ball mills are especially
suited for ne and ultra-ne grinding of hard and brittle material
down to the nanometre size range [1], for mechanical alloying and for
mechanochemical reactions (among others [25]). In comparison to
ball mills and vibrating mills higher stress intensities can be generated
due to the centrifugal eld. The stress intensity describes which
energy the mass of the feed particles caught between the grinding
balls are stressed [6]. High stress intensities and other benets
(simple set-up and handling, cleanability, moderate costs) make
batch operated planetary ball mills very well suited and popular for
application in laboratory scale process development, e.g. in pharmaceutical industry [7].
A transfer problem occurs then, when taking such a newly
developed process to production scale: due to their working principle,
large installation sizes of planetary ball mills show major technical
difculties in the mills' drive systems [8], with cooling of the grinding
chambers in dry grinding and the design of feeding and product
Corresponding author. Tel.: + 49 531 3919621; fax: + 49 531 3919633.
E-mail addresses: s.rosenkranz@tu-braunschweig.de (S. Rosenkranz),
s.breitung@tu-braunschweig.de (S. Breitung-Faes), a.kwade@tu-braunschweig.de
(A. Kwade).
0032-5910/$ see front matter 2011 Elsevier B.V. All rights reserved.
doi:10.1016/j.powtec.2011.05.021
225
dGB
= MGB
dt
mGB
IGB
where mGB, vGB, GB and IGB are the mass, translational velocity,
angular velocity and moment of inertia of a single grinding ball inside
the grinding chamber. FGB and MGB are the forces and moments acting
on the grinding ball, respectively. The most important force acting on
a grinding ball inside a planetary ball mill is the contact force. The
contact force can be generally modelled by a springdash pot system
with friction element. In this work a non-linear contact model based
upon the work of Mindlin [24] was used. It is the so called HertzMindlin contact model provided with the commercially available
software EDEM 2.3 (DEM Solutions Ltd.). The detailed contact force
calculation, as described in Ref. [25], is shown in the following by Eqs.
(3)(12).
The resulting contact force is given by:
n
F = F + F + Fd + Fd
Table 1
Operating parameters of the laboratory planetary ball mill. Standard values for this
study are typed bold.
Fig. 1. Photograph of the experimental set-up with camera xed to the sun wheel.
Camera position is highlighted by a dashed square, grinding chamber positions by a
square.
Parameter
Value(s)
Unit
Speed ratio k
Sun wheel angular velocity s
Sun wheel diameter dS
Grinding chamber diameter dG
Grinding chamber height hG
Ball diameter dGB
Ball lling ratio GB
Feed lling ratio F
3; 2.5; 2; 1
20.9
300
100
72
10
0.3; 0.5; 0.7
0; 0.5
s 1
mm
mm
mm
mm
226
F =
4 p n32
E R
3
Fd = 2
5 p
n
Sn m vrel
6
S = 2E
n
p
R n
t t
F = S
5
6
7
3. Results and discussion
and
3.1. Experiments
t
Fmax = S F
t
Fd
r
5 p
t
= 2
St m vrel
6
t
S = 8G
p
R n
9
10
11
i = jF j R Ri i
12
contact point from the center of mass and i the unit angular velocity
vector of the object at the contact point.
The restitution coefcient e and the friction coefcients S and R
can be determined experimentally via drop tests and tribological
measurements. For this study, model parameters for steelsteel
Fig. 2. Effect of varied speed ratio k on grinding ball motion pattern at low friction (no mill feed added). Top row: experiment, bottom row: simulation.
Value(s)
Unit
10
7800
80
0.3
0.7
0.2; 0.35; 0.5; 1
0.01; 0.1; 0.5
10 6
mm
kg/m3
GPa
227
Fig. 3. Effect of varied speed ratio k on grinding ball motion pattern at increased friction (in the presence of marble powder, F = 0.5).
228
SE =
vrel m1 m2
2m1 + m2
13
Fig. 5. Inuence of different mill feed materials on ball motion pattern, a) no feed, b) limestone, c) alumina, d) marble.
229
Fig. 6. Inuence of varied friction coefcients on simulated ball motion. Standard values
are typed bold, ball motion qualitatively tted to different feeds (compare Fig. 5).
Fig. 9. Inuence of varied friction coefcients on stress energy distributions of
collisions. Simulation was qualitatively matched to ball motion in experiments with no
feed, limestone or alumina and marble (see Fig. 6).
kinetic models. The main reason is the neglect of friction and slip in
these prior considerations.
Different ball motion patterns exist at varied grinding ball lling
ratios, namely with increasing lling ratio cascading over cataracting
to centrifugation.
Furthermore, the grinding ball motion is strongly affected by the
friction arising, among others, from different feed materials. Thus,
friction necessarily has to be considered in studies on stress
conditions in the planetary ball mill. Utilizing a Discrete Element
simulation model, a sensitivity analysis shows that both friction
coefcients, i.e. static and rolling friction coefcients, strongly
inuence ball motion, relative collision velocities and stress energy
distributions. The results fortify the approach to account for mill feed
by changing friction coefcients.
The experimental as well as simulation techniques are currently
being rened to gain further insight to the grinding ball motion as
well as stress conditions and their dependency on the process
parameters in the planetary ball mill. Corresponding experiments
with the presence of feed material have to follow in order to identify
the ball motion resulting in optimum product neness. Other
operating parameters, like geometrical changes, have to be looked
at, too.
4. Conclusions
On the basis of video camera images, no considerable inuence of
speed ratio on the grinding ball motion pattern could be observed in
the range 3 b k b 1. This contradicts older theoretical calculations
given in the literature, where the ball motion was calculated based on
Acknowledgements
The authors gratefully acknowledge nancial support by the
German Research Foundation (DFG). The planetary ball mill was
kindly supplied by Retsch GmbH. Furthermore, support by DEM
Solutions Ltd. within the EDEM Academic Partner Program (EAPP) is
thankfully acknowledged.
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Fig. 8. Inuence of varied friction coefcients on the number of collisions per time and
grinding ball.
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