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ABSTRACT: Considering the eect of bubble-emulsion structures in bubbling uidized beds, a bubble-structure-dependent
drag coecient model is developed. Accelerations in the bubble and emulsion phases are incorporated into the solution of the
drag coecient. Meanwhile, the inuence of solid pressure and bubble-induced added mass force is also taken into account. In
combination with the two-uid model, ow behaviors in two-dimensional and three-dimensional bubbling uidized beds are
simulated. The predictions by the present model with consideration of bubble eects are in more reasonable agreement with the
experimental results compared to the Gidaspow drag model. It is shown that the present model obtains a zonal distribution of the
drag coecient with solid concentration, which reveals that the drag coecient not only depends on the local solid concentration
but also is greatly inuenced by the local velocities.
2014 American Chemical Society 15776 dx.doi.org/10.1021/ie502412g | Ind. Eng. Chem. Res. 2014, 53, 1577615785
Industrial & Engineering Chemistry Research Article
introduced. Compared with empirical relations and exper- T1-7, where g represents the gas viscosity and is assumed to be
imental results, the model agreed well with the available data. constant in the current work.
Wang et al.21 and Lv et al.22 established drag models on the At a high solid concentration, particles are closely packed and
basis of local structures, where local structural parameters are inuenced by sustained contact with multiple neighbors. The
obtained by solving the mass and momentum conservation frictional stress of sliding contacts is dominant. Here, the
equations and empirical correlations of the bubble velocity and friction stress model proposed by Srivastava and Sundaresan25
bubble diameter. The above models used the global hydro- is adopted to consider the frictional contribution, which
dynamic conditions to deduce the correlation between the drag modies the Savage26 model to take strain rate uctuations
coecient and voidage, which neglected the dependence of the into account. The kinetic theory is still used to describe the
drag coecient on the local information in the control volume. kinetic and collisional contribution. To provide a smooth
In this paper, a bubble-structure-dependent (BSD) drag transition between the shear ow and frictional regime, a
model is developed on the basis of the previous cluster- transitioning function is introduced.27 The kinetic and
structure-dependent (CSD) drag model.23 The heterogeneity frictional components of solid pressure are expressed by eqs
within a computational cell caused by bubbles is described by T1-9 and T1-10. The shear and frictional viscosities of the
resolving the overall system into subsystems. The pressure particle phase are given by eqs T1-14 and T1-15.
2.2. BSD Drag Coecient Model. In the previous study,
gradient due to particleparticle collision interaction and the
the CSD drag model was proposed to describe the eect of
bubble-induced added mass force are incorporated into
mesoscale structures in fast uidized beds.23 The local
calculation of the drag coecient. The accelerations in the
heterogeneous ow is resolved into three phases: the dense
emulsion and bubble phases are also taken into account. By phase in the form of clusters, the gas-rich dilute phase, and the
means of two-dimensional (2D) and three-dimensional (3D) interface. Bubbles, as typical mesoscale structures, lead to a
simulations of bubbling uidized beds, the bubble-based drag nonuniform drag solution in bubbling uidized beds.
model can give better predictions of the experimental data. Analogously, the local ow within the grid is separated into
three subsystems: the emulsion phase, the bubble phase, and
2. MATHEMATICAL MODEL the interphase, as displayed in Figure 1. Here, it is assumed that
An EulerianEulerian multiphase model is adopted in the the bubble phase only includes the gas phase and the
present study. The main assumptions of the model are as distribution of particles in the emulsion phase is uniform.
follows: (1) mass transfer between the phases is neglected Hence, the BSD drag force consists of two contributions: one
because of no reaction; (2) the diameter and density of the from the drag component in the emulsion and the other from
the bubble-induced drag component, which is expressed as
particles are uniform. The governing equations consist of the
follows:
conservation equations of mass and momentum. The kinetic
theory of granular ow is used to close the model, as reviewed gFgs g
by Gidaspow.24 Detailed information can be found in Table S1 BSD = = (neFde + nbFdb)
Uslip Uslip (1)
in the Supporting Information (SI).
2.l. Hydrodynamic Model. The continuity equations for where nb and ne are the number densities of bubbles and
the gas and solid phases are given by eqs T1-1 and T1-2 (see particles in the emulsion phase. Fde and Fdb denote drag
the SI). The momentum conservation equations of the gas and components in the emulsion phase and generated by bubbles,
solid phases are expressed by eqs T1-3 and T1-4, where and respectively. Detailed correlations are listed in Table S2 in the
denote the stress tensor and the gassolid drag coecient, SI.2831
respectively. To describe the uctuating energy of the particles, To solve the mutiscale drag coecient, six independent
granular temperature is introduced and dened as = C2/3, parameters are required, that is, the volume fraction of bubbles
where C represents the uctuating velocity of the particles. The (b), the voidage in the emulsion phase (e), the supercial gas
conservation equation of granular temperature is described by velocity in the emulsion phase (Uge), the supercial solid
eq T1-5. velocity in the emulsion phase (Use), the velocity of the bubble
Constitutive relations are used to close governing equations. (Ub), and the diameter of the bubble (db), which can be
The gas and solid stress tensors are expressed as eqs T1-6 and obtained by solving a set of nonlinear equations.
15777 dx.doi.org/10.1021/ie502412g | Ind. Eng. Chem. Res. 2014, 53, 1577615785
Industrial & Engineering Chemistry Research Article
Figure 4. Instantaneous concentrations of particles in bubbling uidized beds: (a) Gidaspow drag model; (b) BSD drag model.
Figure 11. Proles of the solved bubble diameter and number density
of the bubbles with the solid concentration.
Figure 8. Variation of the bubble rising velocity with the bubble
diameter.
Figure 12. Prole of the drag component with the solid concentration.
Figure 9. Prole of the solid pressure gradient and added mass force
with the solid concentration. concentration increases, the accelerations in the emulsion and
bubble phases decrease and tend to zero. The acceleration of
Here, the accelerations in the emulsion and bubble phases with the bubble phase is higher than that of the emulsion phase. This
the solid concentration are shown in Figure 10. The implies that the rate of momentum change in the bubble phase
accelerations in the emulsion and bubble phases are directly is more obvious.
calculated from local independent variables. We can nd that Figure 11 shows the distributions of the solved bubble size
both accelerations display a similar trend. As the solid and number density of the bubbles with the solid
15781 dx.doi.org/10.1021/ie502412g | Ind. Eng. Chem. Res. 2014, 53, 1577615785
Industrial & Engineering Chemistry Research Article
Figure 13. Prole of the drag coecient with the solid concentration. Figure 16. Size distribution of quartz sand particles.
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AUTHOR INFORMATION
Corresponding Author
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