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Received 30 June 2017; revised 9 October 2017; accepted 9 October 2017; posted 25 October 2017 (Doc. ID 300884); published 15 November 2017
Electromagnetically induced absorption (EIA) and velocity-selective transparency peaks are observed in the probe
absorption signal of V-type five-level atomic systems interacting with copropagating control and probe fields.
At high control beam intensity, a splitting of EIA occurs. The experiment shows similar results for both
87
Rb and 85 Rb isotopes at room temperature. A density matrix-based theoretical model of this five-level system
has been developed and solved numerically under steady-state condition. The simulated spectra agree quite well
with the experimental findings. An analytic expression for the probe response is derived and used to find out the
causes for the splitting of EIA. 2017 Optical Society of America
OCIS codes: (140.3460) Lasers; (270.1670) Coherent optical effects; (020.3690) Line shapes and shifts; (080.2710) Inhomogeneous
optical media; (020.4180) Multiphoton processes.
https://doi.org/10.1364/JOSAB.34.002550
2. EXPERIMENT
Figure 1 shows the experimental arrangement schematically.
The probe transmission through an Rb vapor cell containing
87
Rb (27.83%) and 85 Rb (72.17%) is measured in the presence
of a copropagating high-power control (pump) laser field. Two
external cavity diode lasers (both from Toptica Photonics AG,
Germany and having free-running linewidth less than 1 MHz)
operate at 780 nm, one as the pump or control laser and the
other as probe laser. We have used an optical isolator to prevent
feedback of the laser beam from optical components such as
mirrors into the laser diode. In this experiment, the probe laser
is locked to the crossover transition occurring between the
F 32 F 0 32 and F 32 F 0 43 hyperfine Fig. 2. Five-level system resembling the 52 S 12 52 P 32 transition of
peaks of 85 Rb (87 Rb), as shown in Fig. 2. 85 Rb. The dashed lines represent the spontaneous decay paths of pop-
The hyperfine and the crossover peaks of Rb D2 transitions ulation from the excited states to the ground states. The dotted lines
are resolved by a standard setup for saturation absorption spec- represent nonradiative transfer of population between the two ground
troscopy. The crossover transition is selected by properly tuning levels j1i and j2i.
2552 Vol. 34, No. 12 / December 2017 / Journal of the Optical Society of America B Research Article
effects of the stray magnetic fields as well as the magnetic field theoretical analysis, as will be discussed later. The peak posi-
due to the Earth on the measurements. The external magnetic tions have been labeled as a, b, c, d, e, f, and g
field inside the -metal shield is less than 1 mG. We have cal- in Fig. 3, with peak c not clearly distinguishable from the
culated transit time broadening of atoms in our experiment, background. The peaks corresponding to transitions having
which is 0.233 MHz. The laser beam waist is 2 mm. A var- lower strengths are weak and sometimes have inadequate sig-
iable neutral density filter has been used to adjust the intensity nal-to-noise ratio, and therefore cannot be observed clearly in
of the control beam. The polarization of the control and the the experimental spectra. At higher values of control Rabi fre-
probe beams are adjusted in such a manner so that the two quency, it becomes difficult to identify the peak e from the
beams are separated when they fall on the polarizing cube beam background. At lower control intensity, seven peaks can be
splitter placed just after the Rb vapor cell. This allows us to identified, but at higher control field intensity, the smaller
detect only the probe beam with the help of a fast photodetec- peaks get masked due to the power broadening. With the in-
tor (New Focus) [15]. The residual Doppler shift due to the crease in the power of the control field, the EIA signal also gets
possible directional mismatch of the control and the probe laser more and more prominent, and for a control beam Rabi fre-
beams can be neglected in this case [15]. This measurement was quency 33.86 MHz (Fig. 3 and the inset therein), we can
performed in the Laser Spectroscopy Laboratory of Saha clearly observe a transparency-like peak trying to come out
Institute of Nuclear Physics, Kolkata. of the EIA background. There has been an earlier report on
the conversion of EIT into EIA in a -type system [14]
3. EXPERIMENTAL RESULTS and N-type system [19]. Kim et al. [16] observed EIA to
The schematic of the five-level system is shown in Fig. 2. Here EIT transformation in Cs-D2 transition by varying the pump
the probe laser is kept locked to the crossover signal appearing beam power. They measured the probe absorption spectrum by
between the F 3 F 0 3 and F 3 F 0 4 hyperfine changing the probe detuning. In our experiment, similar behav-
peaks of 85 Rb. The spectra were recorded by a digital storage ior of the probe response has also been found in the case of Rb
oscilloscope by scanning the pump laser frequency from the vapor with control field scanning. The appearance of the EIA
F 3 to F 0 2; 3; 4 hyperfine levels. Thus, an effective signal and splitting of the EIA peak is clearly visible as we keep
five-level system is formed, where the population from the on increasing the value of the control field intensity. We have
upper levels F 0 2; 3 are allowed to decay spontaneously to tried to understand the physical phenomena of the conversion
both of the ground hyperfine levels j1i and j2i (F 2 and by detailed theoretical simulation numerically and analytically.
3). But the selection rule allows spontaneous decay of popula- The EIA signals corresponding to different values of control
tion from the uppermost excited state (F 0 4) to only the Rabi frequency are fitted with a Lorentzian line profile, and
upper ground level j2i (F 3) and not to the lowest ground only those EIA signals are used for this purpose, for which
level j1i (F 2). Since the lowest ground level is not coupled no signature of the splitting is present. The values of the fitted
to any other excited states by the applied laser field, population full width at half-maximum (FWHM) of the EIA signals
that decays to this level has only one way to come to the upper are 3.63 MHz, 3.81 MHz, 4.25 MHz, and 4.33 MHz,
ground level in this scheme, and that is through collision. We corresponding to control Rabi frequency of 13.18 MHz,
have performed the measurements on both 85 Rb and 87 Rb. 16.14 MHz, 22.83 MHz, and 25.01 MHz, respectively.
Figure 3 shows the probe response signal of 85 Rb, which has The widths of the EIA signal are found to vary linearly with
six prominent VSTPs, with one of them carrying a signature the control Rabi frequency, as shown in Fig. 4 for the 85 Rb
of EIA. There should be seven such peaks according to our atom. The width of the EIA signal is much less than the natural
linewidth of the transition, i.e., 6 MHz, so we observed
subnatural EIA linewidth. A plot of the zoomed VSTP peak of
q
S
jji (with j 3, 4, 5 here) is ij 3ij jhJjerjJ 0 ij, where
S ij is the relative hyperfine transition strength factor [8].
p
J 12 and J 0 32 here. Rabi frequency is defined as 2j
p E
S 2j p with p pp jhJjerjJ 0 ij. E p stands for the ampli-
3
tude of the applied probe laser field. The ith level population is
ii (i 1, 2, 3, P
4, 5 for this level scheme) with the normali-
zation condition 5i1 ii 1 [15]. ij (i j, i, j 1, 2, 3, 4,
5) are the off-diagonal density matrix elements, which are also
known as the coherence terms. For this five-level system, a total
of 25 optical Bloch equations [22] are derived by using the
Liouville equation, where the phenomenological decay terms
are added. The coherence terms 2j (j 3, 4, 5) [22,23]
can be written as follows:
Fig. 5. Plot of zoomed VSTP signal of 87 Rb versus control field X5
p
X
5
detuning (c ). The occurrence of the transparency peak at the higher 2j 2j e ip tkp z c2j e ic tkc z : (3)
j3 j3
value of the control Rabi frequency (c ) is clearly visible.
These terms have contributions from both the control field and
the probe field. A set of optical Bloch equations under steady-
87 state condition (i.e.,
t 0) is given below. The complex
Rb, over which the EIA signal and its splitting are visible, is
conjugates of the equations are not shown:
shown in Fig. 5. The reason behind the formation of the seven
VSTPs is explained in the next section. A similar situation was 12 11 21 22 31 33 41 44 51 55 0; (4)
encountered earlier while studying a six-level -type system
[15]. We shall explain this for 85 Rb in the following section; ic23 c ic ic
the explanation for 87 Rb will be identical. 32 c23 24 c42 c24 25 c52 c25
2 2 2
p p p
i p p i p p i p p
23 32 23 24 42 24 25 52 25
4. THEORETICAL MODEL 2 2 2
We explained these experimental results by a proper theoretical 12 11 21 22 32 33 42 44 52 55 0; (5)
model to find out how VSTP peaks are generated and how
p
splitting of EIA occurs with increasing pump power. Now ic23 c i p p
23 c32 23 23 32 31 32 33
we are going to describe the theoretical model for the five-level 2 2
system (as shown in Fig. 2), interacting with two copropagating 43 44 53 55 0; (6)
laser fields. In our system, both the control and the probe fields
are allowed to connect all the excited levels j3i, j4i, and j5i ic24 c i
p
p p
from the common ground level j2i (see Fig. 2). These cou- 24 c42 24 24 42
2 2
plings make our system different from a conventional system,
where the control and the probe fields act on different levels. 41 42 43 44 54 55 0; (7)
The total Hamiltonian of the system can be written as p
H H0 HI , where H0 is the unperturbed Hamiltonian, ic25 c i p p
25 c52 25 25 52
and HI represents the interaction Hamiltonian [21]: 2 2
X
5 51 52 53 54 55 0; (8)
H0 i jiihij
i1 ic23 ic ic
32 ic32 c32 33 22 24 34 25 35 0;
1 j1ih1j 2 j2ih2j 3 j3ih3j 2 2 2
4 j4ih4j 5 j5ih5j; (1) (9)
p p p
p p i24 i i
42 i42 42 44 22 23 43 25 45 0;
2 2 2
(12)
ic25 ic ic
52 ic52 c52 55 22 23 53 24 54 0;
2 2 2
(13)
p p p
p p i25 i i
52 i52 52 55 22 23 53 24 54 0;
2 2 2
(14)
Fig. 6. Plot of simulated probe transmission versus control field
p p
ic i p ic i p detuning (c ) for 85 Rb. In the inset, the zoomed probe transmission
43 i43 43 23 c42 23 42 24 c23 24 23 0; is shown around c 70 MHz. The values of the control and probe
2 2 2 2
field Rabi frequencies are mentioned in the figure.
(15)
acting behind the formation of the VSTP signal and the spac-
ings between the VSTPs for 87 Rb [13]. Because of the differ-
ence in the hyperfine separations between the two isotopes, the
velocity groups of atoms interacting with the coherent radiation
fields would be different for 87 Rb. It is also to be noted that only
for Fig. 7(iv), both the pump and the probe fields are sending
the same velocity group of atoms (namely 39.41 ms) from
F 3 ground state to F 0 4 excited state, i.e., Fe Fg 1
(Fg > 0), where Fe and Fg are the total quantum numbers of
the excited and ground states, respectively [24]. This is a close
transition, according to the selection rule. The polarizations of
the probe and the control fields are linear but orthogonal to
each other. This leads to the formation of EIA due to transfer
of coherence (TOC) [24]. We have shown the simulated probe
transmission spectra versus control detuning for 87 Rb in Fig. 8
for four different values of control Rabi frequencies. The split-
ting of the EIA signal in the background of the VSTP is noticed
Fig. 7. Schematic showing the origins of the VSTP signals. The clearly as the pump Rabi frequency is increased (27 MHz and
positions of the control and the probe fields corresponding to the peak above). The simulation is in agreement with the experimental
positions a, b, c, d, e, f, and g of Figs. 3 and 6 are shown observation (Fig. 5).
in (i)(vii), respectively. To understand the splitting in the EIA signal at a high value
of control Rabi frequency, we have derived an analytical
expression for a three-level V-type system from the set of
(52 S12 F 3 52 P32 F 0 2 for 85 Rb). Thus peak a in Figs. 3 density matrix equations presented earlier. Here we consider
and 6 appears. Similarly, when the pump beam is detuned by one ground level (j2i) and two excited levels (j4i and j5i)
50.64 MHz from level j4i [Fig. 7(ii)], it again comes to reso- (see Fig. 2); control and probe beam couples both the excited
nance with the same velocity group of atoms and sends them to levels, and all population is in the ground state when no field is
j4i from j2i (52 S12 F 3 52 P32 F 0 3 for 85 Rb), thereby cre- present, i.e., 22 1 for simplicity of the solution. The
p
ating the peak b in Figs. 3 and 6. The separation between the approximate analytical expression of 52 , obtained under a
peaks a and b is 1 63.40 MHz. The pump beam then steady-state condition by using perturbation technique, is given
reaches the position shown in Fig. 7(iii), where it is blue- below. We have retained the terms containing probe Rabi
detuned by 70 MHz with respect to level j3i, and hence frequency up to the second order and also assumed 22 1:
pumps the atoms having velocity 54.47 m/s. This is the reason Z p
i25
p
behind the appearance of the peak c in Figs. 3 and 6, 52 2
p2
M vdv:
although it is masked by power broadening. The strengths
p 24
ative strengths of the associated transitions from j2i to j3i and (19)
j2i to j4i compared to the transition from j2i to j5i. Thus, we p
see that the relative strengths of the hyperfine transitions from In Fig. 9(A) we have plotted the imaginary part of with 52
the same ground level do play an important role in the forma- control detuning for different values of control Rabi frequency
tion of VSTPs. The pump beam then reaches the position of
the locked probe beam [Fig. 7(iv)] and becomes on resonant
with three different velocity groups of atoms simultaneously
and excites them to the three different levels j3i, j4i, j5i from
the ground level j2i. This affects the probe absorption, result-
ing in the strongest of the VSTP peaks (d in Figs. 3 and 6).
The separations of the peaks a, b, and c from d are
1 2 , 2 , and 1 , respectively, where 1 and 2
are the separations between the upper hyperfine levels
(j3i j4i) and (j4i j5i). Similarly, the peaks e, f, and
g of Figs. 3 and 6 are created when the pump beam reaches
the positions given by Figs. 7(v)7(vii), respectively. It interacts
with the 88.74 ms, 54.47 ms and again with
88.74 ms, respectively, to pump them to the levels j4i
and j5i. The separations between these peaks are just similar
to the peaks appearing to the left on these spectra. A similar Fig. 8. Plot of simulated probe transmission of 87 Rb versus control
argument can be used to describe the physical mechanism field detuning (c ).
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