NUMBER 2 JANUARY 15, 1959
Lifetimes of Nuclear Isomers*
Srovex A, Mostxowsxit
Unisersity of Chicago, Cheap, Minos
(Received August 29, 1952)
Lifetimes of muclaa isomers for gumma-teansitons are caleu-
Jated theotetially on the basis of various independent particle
models; single proton, single neutron, and states of several
particles (Sec. I}, The eaiulatons of this paper are etentially|
Festricted to the mnst common type of transition ws, multipole
‘eder equal to spin change. The lifetime is expresod in terms ofa
‘matrix element, AF, whose theoretical value depends on the
particular made of the nucleus, Radial integrals are cleulted
‘umercally, assuming that the nuclear wave functions aze given
by single partile wave funetions fora sphetieal square well
"Bmpirical values of MP can be deduced from measured isomer
Ifotimes corected for internal conversion, An analysis of et.
pirical AP for some gamma transitions points to. number of
‘egulartes which, in general, speak in favor of an independent
partele model (Se. 11D.
"The regularities are the following:
Enel values of A for AP transition are of order unity nd
show litle scattering and no distinction between edd proton and
fold neutron auc, The lack of scattering within each group of
transitions 1s consistent with predictions of a single particle
1. INTRODUCTION
Twas first suggested by v. Welzsucker,! and has
become generally accepted, that nuclear isom
states decay into each other by gamma-emission, but
that the lifetime is large ifthe spin of the two states
differs by several units of
The emitted quantum may carry off angular mo-
mentum L(21), giving rise to electric or magnetic 2"
pole radiation (denoted in this paper by EL or AF),
according to whether the quantum has parity (—1)¢
or (1) Te follows that the selection rules for BL
and ML radiation, i.e, radiation of various multi
polatities, are
WL] SLE, a
parity change (—1)4 for EL, (—1)!' for ML. Here I,
and J, denote the spins of the initial and final states,
respectively.
Electromagnetic radiation is not the only mode of
decay for a nuclear excited state, Instead, an internal
conversion electron may be emitted; ie, an orbital
electron may be ejected and carry off the energy of
excitation. ‘The number of electrons emitted from a
given shell per quantum is called the conversion coef-
ficient for that shell. Values of conversion coefficients
depend on the multiplarity ofthe transition and on the
clectronie configuration. However, they do not depend
fon the detailed structure of the aucleus, and can
* This work was caved out i partial flfllment ofthe require
ments for 8 PRD. degre at the University of Chicago. 1 was
erted by an AEC Predoctoral Fellowship.
Now at Columbia University, New York, New York
ICR, Welzsacker, Natur, 24, 813 (1980).
‘model. However, according to this model, one would expect odd
proton auc to have lifetimes about hal as large as odd neutron
heli forthe same transition energy, and also would expect life
tines about 1/10 as large as found empirically. Empirical values
(of BF for 444 transitions appeer to be larger for transitians In
‘nuclei with neary closed shel
“According to an independent particle model, 3? for £3 tans
tions of energy 100 key shouldbe of order 10 for single neutron
tuanstions, and vanish for many particle transitions, such as
‘those between py and 7/24-states. The fact that empivial 30
{or £3 transitions are small can be interpreted as resulting from
small deviations fom an independent particle model. In fact,
empirical A for transitions between py and 7/2-rstates in od
feutron nuclei appear toe emailer the more nearly the nucleus
an be represented asa closed sell nucleus.
“The empirical value of for an M01 isomeric transition in Li?
is slightly larger than expected according to an independent
particle model
“A graph of energy levee fo
presented (Appendix, Fig. 2).
pherical square well potential is
therefore be calculated, in principle, to the same ac-
curacy as spectroscopic problems.
‘Keconversion coeficients have been calculated by
Rose el al? neglecting the effect of screening, for
energies above 150 kev, and by Reitz for selected cass,
including the elfect of screening. Calculations of K, Lay
La and Lau conversion coeficients over a wide range of
energies and including screening effects aro now in
progress. -
Conversion data are extremely useful for obtaining
rmultipolarity of a transition, but not for obtaining
information regarding detailed nuclear structure (apart
from thespin and parity change). Goldhaberand Sunyar*
have made mulipolarty assignments for many transi
tions by comparing observed K-coeficients with Rose's
theoretical values, and. also from a. semi-empirical
analysis of K/L ratios, which indicates that K/L. ratios
are a function of 23/2 and multipalarty alone (except
for ¢1 transitions). The work of Mibelich and Church?
indicates that ratios of L-subshell conversion coeficients
can be of use for assigning multipolarities and for
analyzing transitions which involve a mixture of
rultipolarties.
‘The lifetime of an excited state for gamma-emistion
depends not only on the multipolarity and energy of
the transition, but also on the detailed structure ofthe
nucleus. Its, thus, not possible to identify the multi-
7 Rowe, Goerte, Spinrad, Harr, and Strong, Phys. Rev. 88, 1
st)
1 it, Reitz, Phys, Rev. 77,10 1950).
'E- Rosé and G. Goetze (o be publlsed),
SME Galdhaer and A-W. Sunyar, Phys. Rev. 88, 906 (1951),
ME Goldhaber (private communication)
1 T'WeMibelch and FL, Church, Pays, Rev. 85, 738 (1982);
J..W, Mrinal, ‘Phys: Rev. 87, 646 (1933)
44polarity of a transition from a lifetime measurement
alone, without specific assumptions as to nuclear
structure,
However, information regarding nuclear structure
can be obtained by comparing the measured lifetime of
a transition with the lifetime calculated using a specific
nuclear model, eg, the independent particle model,*
provided the multipotarity of the transition has already
been identified, say, from conversion data,
U, THEORETICAL CALCULATIONS OF LIFETIMES
"FOR GAMMA-DECAY
4. Single Proton for Spin Change Equal to Multiple
Order-Central Potential
The transition probability per unit time for a system
to undergo an electromagnetic transition from an initial
state ¢ to a final state / is given by the wel-known
equation®
an
Wa sey! 46) 2
7 . @
Here 5¢y is the matrix element of the electromagnetic
interaction between particles and field, (B) is the
number of final states available per unit energy interval.
‘The total nonrelativistic Hamiltonian of proton and
clectromagnetic field can be written'®
tN arate H+E mbes
@
Here A denotes mass of proton, ur is the proton mag-
netic moment in nuclear magnetrons. The vector
potential, normalized to one quantum per unit volume
is given by,
@
‘The radiation interaction is contained in (3) and is
given by
Am e(2ehct/)tems,
e oh
@
[The term (c/2M@)A is neglected here, as are second
order perturbation terms, both of which give rise to
double quantum emission, with a transition probability
which is usually several orders of magnitude less than
the transition probability for single quantum emis-
sion. }** The first term in (S) is the interaction energy
of a point charge with an electromagnetic field, while
the second term is the interaction energy of an intrinsic
magnetic moment with the field. The transition prob-
ability between states is calculated using (2), summing
YM. G, Mayes, Phys. Rev. 78, 16, 22 (1950)
HET Sthnde Quantum echander (McGraw HE Book, Com
vag igaNe Fon 9 ale
Wile The Quantum Theory of Radiation (Oxford Uni-
vepiy Be Landon 8), on 3
oeppert Mayer, Ani Phyit 9, 273 (930,
RG Sach Page ev. 87, 198 940,
FETIMES OF NUCLEAR ISOMERS
415
over polarizations, and integrating over all directions
of emission:
Seva (O)
he
Here dQ, is the solid angle for direction of emission,
o
(