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32,r29
32,r30 TROSNIKOVAND NOBRE:AEROSOLTRANSPORTFROMBÌOMASSBURNTNGAREAS
Figure 1. GOES-8 r.isiblcimage of sniokc c:onr:cntr:rtion (n) at 1145UTC, Augrrst 20, 1995.arrcl
( b ) a t 1 1 4 5L Ì T C . , \ r . r g r r s2t 9 , 1 9 9 5 .
r,ahrcs are ttsecì. Tht: r'aluc of tÌlc tlactlr ts st''t trtluaÌ ttl b1' sources and tÌre âerosol fllrx through the late-:..-
-
zcro for arrival poiÌÌts lor:atc<i btllou' tÌtrl srrrfactl oí thtl Ìrounciarl'consequcrrtÌyon the time intcrval (/ - ll.
E:rrtÌr.
tr: - Àt)p(r- Lt)rlrrt'uttz t
l,x't'(l
3. Conservation
A conserr,atiorr lry usirrg
aÌgorithrnltasÌtectlrlt:sigrrctÌ c -z,: Lt I srara'uaz i-
icle:rsfrorn thc fltrx-correttttt:dtlattsllort (FCT) rricthocl Jv
trartsport equa-
lPrze.stl,rry,1993] . The solutiolÌ of tÌtc f ..
C,,: f Í l,t'" ir lÍ)nv(ú - ^l)dÍ), (12
tion for eaclt poirrt rvitÌt itrcÌtlx À: is rlÌltaitretl frtlrtt tu'<'r ./,
apploxirnatirltrs of tltc: sttirtl,irltl at tlrtl tttln' tilrle 1evtll.
n is thc insiclt:rrorrnalto tÌ'relatcraÌ borrrttlarv0. Wherl
tÌre hìgÌr-orrÌcr soltttiott, 1fJ. tlÌrtainelcl lrv cr.tÌ;itlinter-
tire sources :rncl flr.tx throrrgh the latcraÌ Ìloundary are
polatiorr, and tÌrc lol,-order sttlirtìon, 1f , obtainccÌ bv
aÌrsent,tÌrc rnass of aerosolis cortservationvaÌue. The
Ììncar intcrpoÌatiott,
Priestkrt' aÌgorithrn is used for cleterrnirrationof a6 br'
\ 1 1: . t r . r [ I * ( t - r r 1 ) 1 f r (6) rnirrirnization of the clifl'erenccÌretrleen 1Àí ancl 1H n'itÌt
c o n c l i t i o n( 8 ) .
0(rip(1 (7)
u'liere crÀare to Ìrc <thosensrrr:Ìras to rrrakethc conser 4. Simulation of Aerosol TYansport
vative scherneÍbr vohrrrie l'
for SCAR-B Experiment
I
L , \' r(,l ' l P ( t1 t l ' r t l t l t=l . (' ,
For tÌic sirnulation of aerosoÌtranspclrt, the anaÌysis
(8)
I r
,J \:
ficlrlsof tÌre u,ind. teÌnperatlrre,arr<lgeopotentialheight
q'herr:r'nÌue C includcs thc tÌrrec tcrms procìucerri Ìrv tlic CPTtrC gÌobaÌ nunr:rical q'eather fore-
<:astrnodcl and avaiÌabÌe from SCAR.-B clatabaservere
C:Ct+Cz*Ct. ( 9 ) usecl.Thc grid of the anaÌ1'ses has 49 x 41 points rvith a
horizontaÌ resoÌutionof 1.87õ"x1.875oarid coversSoutÌr
C1 is the aerosoÌtrrassÍbr 1he tirtrc ÌrÌorÌÌetìtt - ^t. C2 A r n e r i c aÍ ì o n i 1 0 1 . 2 5 o \ Vt o 2 6 . 2 5 ' W a n c lÍ ì o m 6 0 o St o
ancÌC: arc tlie eLcrosoÌ
ma,ssinjectecÌin the atniosphere 15'N. Thc transport model has thc lurrizontaÌgrid colo-
TROSNIKOVAND NOBRE:AEROSOLTRANSPORTFROMBIOMASSBURNTNGAREAS
(o)
1.7
t<
1.2
0.7
0.5
na
r / ,/,,'-
0.1
t/.,
-
1,7 1,7
1.5 1.5
1.2
1 1
0.7 o.7
0.5
0.J
0.í i:!Jo.t
_rí _ïo_
cated with tÌre anaÌysesgritl, anrl its vertical structure rvhere AP is tÌre thickness of the air Ìaver with the
includes 22 pressureleveÌsfrom 1000 to 200 hPa, 16 of source in hPa, :rnd g is thc gravitationaÌ acceÌeration.
which are placed in the Ìayer 1000-700hPa. The time The choice of AP Íbr numericaÌ experiments was de-
integration of the rnodel 'lvascarried out with a t hour termined by SCAR-B data, which shou's layers of higÌi
time step, and hourly valucs of the meteoroÌogical eÌe- aerosolconcentrationsat 1800-2500m aÌtitude lArtaro
ments rverecalcuÌatedby linear irrterpoÌation. et a|.,1996].
The aerosolmeasurementsduring the SCAR-B exper-
4.1. Location of Aerosol Sources in Separate iment show that acrosol particles have a size distribu-
Regions
tion with a masspeak at about 0.3 pm diameter lArtaro
The sourcesof the aerosol,S(r, y, z) were set in the et al.,1996). It allows one to use the buÌk representa-
grid points and were defined by two parameters: the tion of aerosoÌparticles for transport calculations as the
interrsityof the aerosolinjection to thc atmosphere56(g first approximation. The velocity of the sedimentatiorr
--2 s-t) and tlie totai thickness of the source layer rvas taken to be 0.001 ms-L et al., 1991a]ac-
lPen,n,e'r
AP(hPa) . The simple verticaÌ changesourcemodel was corclingto this approximation. Becausethe calcuÌations
Ìlsed: s _ g,9o were carried out for a dry season,wet scavengingis not
( 1 3 ) included in the source.
p 1004P'
TROSNIKOVAND NOBRE:AEROSOLTRANSPORTFROMBIOMASSBURNINGAREAS
26/08/es 2s/08/s5
.g
.9
T
Longitude Longitude
The preÌiminary computations sÌrowcdthat the term Tire first simulation of thc aerosol spreading fro::.
of horizontaÌ rrracrodiffrtsion in equation (1) lcads to four separate fire regions during thc period from Au-
a marked increasc of the aerosol spreaclingarea. For gust 20 to 29,1995, is clcrnonstrated(Figures 2 and 3
this reason the simulation of acrosoÌtransport for thc The centers of the regions rvere placed at the poin-'
SCAR-B experiment was conductedu,'ith Ku :0. w i t h c o o r d i n a t e s( 1 ) 5 6 o W , 9 . 5 " S ( t h e r e g i o n o f A Ì : .
In the first numcrical experlrnentsthe foÌlowingsource Floresta); (2) 52"W, 18.5'S (between Campo Granci.
parameters were used: ÀP : 162.õ hPa or the source and Brasília); (3) 55'W, 17'S (betweenCanrpo Grande
height u'as about 1500 2000 m, So:7.5 x 10-6 g rn-2 arrd Cuiabá); and (4) 48.5"W, 13.5"5 (between Portc
s-1. NacionaÌ and BrasíÌia). TÌre initial coriditions for the
To Ìink,9s u,'ith Sy, the interrsitv of thc aerosoÌin- srnoke concentratiorÌ \,'ere set quasi-utriformÌy rvith the
jection to the at,mospliereÍ}orn a firc tcrritory with the averageciensityin tÌre atrnosphericcoltrmrt about of 0.0t,
area Ay, the relation g m-2 anrÌ the geograpÌricconfiguration subjectively ex-
tracted from the GOtrS-8 visible irnageat 1145UTC or.
S o A s: S7A1 (14)
August 20, 1995 (seeFigures la nnd 2a). As shown ir.
can be used, where An is the modeÌ grrclceÌÌ area. For Figurcs 2a and 2b, from August 20 ï,o 23,1995,initiallt'
example,for ^9y:6.993g rn-zs-1 lPe'n"nerel al., 1991b] the sirnulated acrosoÌmoved westerll' from the AIta FIo
a n d Á n - 4 1 5 0 0 . 0 k m 2 , t h e f i r e a r e ai s Á / : 1 0 3 . 8 k m 2 . resta region and southerly from northern Paraguay. B';
TROSNIKOVAND NOBRE:AEROSOLTRANSPORTFROMBIOMASSBURNINGAREAS 32,r33
rìì
15N
10N
5N
500
EQ
5S 400
10s
IJJ
300
20s
200
25S
JOS 1qn
i5s
40s 100
45S
50s
55S 10
60s
5N 500
EQ
5S 400
10s
300
155
20s 204
25S
JOS 150
J5S
40s 100
45S qô
50s
55S 10
60s
90!v 80w 70w 60w 50w 40w 30w 20w
Figure 4. CumuÌatir,eu,eerkÌJ' of fires in the modeÌ gri<l ceÌÌs (a) Íbr Ar.rgust18-24,arrd
rurrrrÌrr:r
( b ) Í o r A u g u s t 2 r 1- 3 1 , 1 9 9 õ .
August 29 it reached35'S" The ÌocatÌonsof tlie cliffer- Thc verticaÌ structure of thc southerlysimulatedaero-
ent aerosolsolrrces:rrc better seen in Figttre 2b. AÍïer sol currents can Ìie seenin the verticaÌ crosssectionsof
August 23, 1995,the sirnulatc<laerosoìbcgatrto spread the aerosoÌconcentratioriaÌong 25'S in Figure 3. Figure
southerly Íìom tÌrc Cuiabii rt:giortattclfortucd a rÌârÌo\v 3:r shou'sa cÌosssectioriof the sirnul:rtcrlacrosoÌcurrent
current which arrivecìat thc ìatitudc bcÌt of 30"S-35"S r,vhichirrcluciesaerosoÌ particÌcs from the Rarrdonia re-
( s e eF i g u r e 2 c ) . gion. In Figure 3Ìr one can scc tÌte aclditionaÌsimuÌatcd
7) l?L TROSNIKOVAND NOBRE:AEROSOLTRANSPORT
FROMBIOMASSBURNINGAREAS
't000
500
N
S Joo
250
200
ffi'oo
,tlil
.,o 150
100
50
10
1000 1000
500
250 250
200 200
150 150
100 100
50 50
10 't0
2A 2C
Figure 5. Sirnulatecliierosol<:oncentratiotr (p,g--3) and wind (- t-t) at 850 hPa: (a) August
20, 1995 (initi:rÌ coriclition);(b) August 23, 1995; (c) August 26, 1995;rind (cl) August 29, 1995,
fbr tÌre experiment rvith loca,tionof the aerosolsourcesin the burning aÌeiìs.
aerosolcurrcnt from the Cuiabri regiorr.Figures 3c :r,nd been useclfor the dctcrmination of aerosol sourcesrr
3d sÌrou' the evoÌrrtion of thcsc sirnuÌatcd itctrosolcur- the model grid points
rents. On account of seclimcrrtation,acrosoÌparticlcs
5 QS,
Ìiave the rìarkc(l rcclistributiori of heìghts clr:pernding
on : (1õ
their Ìifetime in thc atmospherc. , furr'(À,tp,t).
2 6 /0 8/e5 2e/08/s5
15N
10N
e * \ t rt \\\ *
:S\\\ç-Ê-G-ee
$-1r-ê ê í\ Í\ Ê
i
i\À
\ \ \ \ t- \ *
rFÉ\ E **--
"-.-
\{ ( À ì f \
rl-tt/r\\Ì
\ | { t | Ít
\v I
'
\\\'//
\\ .y' t
n t / n, \
-
20
scatterirÌgaÌbedo) in regionalÌrazesin BraziÌ cluringthe agreement with the observcciÌraze on GOtrS-S r'isibÌe
SCAR-B expcrimerit lRe.itlet ol., 19g6]. Figure 7 shows image (seeFigure lb). However,the agreementof tÌrc
the estimatedoptical depth of tlic :rerosolfor Arrgust29, calculated and observed vaÌues of thc optical depth for
'n'aÌrres
1995. TÌic r:tiÌcuÌatec1 are sirniÌitr tcl tÌre vaÌues of locaÌ points is not so good. Tablc 2 shou,sthe (1) modeÌ
the obscrvations Íbr bioniass ilrrnirrg pcriocls lKo,ut',ma,n,estirnated ancÌ (2) obsert'ed optical rÌcpth for the threr.
et al., 19921.TÌre calcuÌatcrÌÌargc-scakrpattcrn of the stations. TÌre obsen'ccl data have becn taken from the
aerosolclistributiorrfor Aupiust 29, 1995,sÌiowsa good AtrRONET (Aerosol Robotic Nctu'ork) data archive.
August 1995
Station 22 23 24 25 29
Alta Floresta
a 1.30 0.95 0.83 0.95 1.11 7.20 7.20 7.32
b 1.18 1.88 1.13 1.11 7.72 1.26 1.30 7.34
Brasília
a 0.04 0.04 0.04 0.02 0.02 0.02 0.03 0.02
b 0.08 0.08 0.08 0.07 0.06 0.08 0.09
Cuiabá
a 0.06 0.13 0.16 0.09 0.09 0.11 0.12 0.16
b 0 . 1 1 0 . 0 4 0 . 1 2 0.06 0 . 7 7 0.08 0.37
The a is model estimated and b is observed optical depth values.
TROSNIKOVAND NOBRE:AEROSOLTRANSPORTFROMBIOMASSBURNINGAREAS 32,137
Although tÌie optical depth Ìer.el rvas simuÌatccl cor- o,t th.eFortaleza, Braztl, Workshop, edited by V. W. J. H.
rectly for the stations, tlierc is a cÌiscrcpa,ncv between I{irchhoff, pp. 9-14, Transtec, São .Joseclos Carnpos, São
estimated a,nclobservcdsm:rÌloptic:rÌclepths.It rnay be PauÌo,Brazil, 1996.
Berrnejo, R., A. Staniforth, The conversion of senii-Lir,gran-
linked rvith the Íbrrrration of aerosoÌrÌensitv for Brasíli:i
gian aclvcctiorrschemesto rlrasi-monotorre schemcs, Mo,n.
arrclCuiabií stations by locaÌ srnall-scaÌcsolÌrcesduring Weo,therReu., 120, 2622-2632, 1992.
August 22-29,1995. Brasseur, G. P., and S. Madronich. Chernistry-transport
moclels, in Cl,imate System Mode.I,íno,editcd by K. tr.
Tremberth, chap. 15, Cambridge University Press, New
5. Conclusions York, 1992.
KauÍman, Y.J., A. Setzcr, D. Ward, D.Tir.rrre,B. N. Holbcn,
The transport rnoclcl Íor tÌrc estintatirtriof traccrs P. \,Ienzel, N{. C. Pereira, and R. R.asrnussen,Biomass
Íïorn biornass burning arc:rs Ìras beerr dcveloped on the Burning Airbornc anrì Spacebornc Experimcnt in thc Ama-
basis of the scmi-Lagrangiantcchnique. The model in- z o n a s ( B A S E - A ) , , / . G e o y t h y s .R e s . , 9 7 , 1 4 , 5 8 1 - 1 4 , 5 9 9 ,
clu<lcsprincipal processes',vhicÌrÍorrn large-scaÌetraccr 1,992.
N,ÍcDougÌ,D., Smoke, Cìouds and Radiation-Braziì (SCAR.-
-preading for cÌrv season: hclrizoritaÌarrclverticaÌ acÌver:-
B) field cxperiment, August 16 to Scpternber 14, 1995,
riorr, sedintentationof aerosoÌparticÌcs, and horizontal \,,Iission Plan, preparcd by SCAR-B scientists and the
rirrbuìcnt excha,nge. No I'erticaÌ cÌiflusiorris incÌurìed SCAR-B Project Oífir:c,N,4.9,4, spec. pu,b\,.,164pp., 1995.
Ln the nrodel ber:ausepoor boundart' Ìa.verlarge-scaÌe Petrncr,,I.E., S.J.Gh:rn,:inrì J..J.Whlton,TÌrc rolc of biorrass
Ìxrrrring in thc budget arrd cycle of carbonaceous soot
IrnaÌysisdata have been rrscdfor aerclsoltransport com-
aerosols and their climate impact, Á Global Biornas.s
:,rrtiLtiorr. They cìo not make it possiblc to estirnatc Burn'ing: Atrn,ospÍteri,c, Cl'rrnate, and B'iosplt,eri'cIrnpli-
;ood parameters of thc corivoctivcborrnclarvlayer. In cat'ion, edited by J. S. Levinc, pp. 387-393, MIT Press,
:act, Íbr burning arcas thc verticaÌ turbrrkrnt cxr:Ìrangt: Cambridgc, Mass., 1991a.
l'as acideclin the transport moclcl bv :r source term Penner, J.tr., NÍ.N,I.Bradlcy, C.C. Chuang, L.L. Eclx''ards,
and L.F. R.adker. A nttrncricaÌ simulation of the acrosol-
equation (15)) which includesfulÌ cornpÌexsubgrid ver- cloud interactions ancÌ atÌnosp}Ìeric clynamics of the Hardi-
rir:iiÌ transport frorn the surfaceto tÌre atrnospÌiere. TÌre marr Township, Ontario, prescribed burn, in Glottal Br'o'
:rrocleÌhas the property of tracer ÌÌìasscorÌservationthat rnassBu,rnzn11:Atrnospheric, Clirnate,,and Biosçtheric Im'
lcrrnits its use for baÌancecalculations. 7tl,ico,t'ion,editecÌ by J. S. Levine, pp. 420-426, NÍIT Press,
Carnbridgc, Nlass., 1991b.
The simulatiorÌ of tlÌc acrosoÌspreacìingfor the SCAR-
Priestlev, A., A quasi-r:onservative vctrsion of the serni-La-
i3 periocl Íïorn August 20 to 29, 1995, sÌrou''erÌtÌr:it the grangiarradvection scherrrc,Mon. WeatÌtlr Rett., 121,62L-
;iir mass locateri beÌorv2 km moveclrnainÌy tcl tÌre south 629. 1993.
irrrclcarricrl thc smokeurrtil 30'S. A slniiÌar tr:rnsport of R,eid, J. S., P. V. Hobbs, and R. J. Ferek. PÌrvsicaÌ and
rìrc aerosolis observccìorr the GOES-8 satellite images. chemical characteristics of biornass Ìturning aerosols in
Brazil, in SCAR.-B Procced'ings:Collection oJ Papers at
.{nother significant transport of aerosoÌ n'as Íi'om the
tÌte Fortalezo,, Brazi), Workshop, editecl bv V. W. J. H.
-\1ta Floresta rcgion to the nortÌrrvest. Kirchhoff, pp. 165-169,Transtec, Sã,o,Josedos Campos,
AlthougÌr thc rrrodeÌ seernsto Ìravr: reillisticalÌy cap- São Pau1o,Brazil, 1996.
turcd the geographicaÌdistribution of aerosolemanat- Staniforth, A., and J. Côté, Serni-Lapirarrgian scÌremesfor
ing from biomassburning areasduring SCAR-B, it stilÌ atmosplrericmodels A revierv, Mon. Weather Reu., 119,
rreecls irnprovementto rcprcsentthc cluarrtitativedistri- 2206-2223, r99r.
Williarnson, D., :rnc1P.Rasch, Two dirnensional semi-La-
Ìrution of opti<::rldcpth. gr:rngian transport lvith shape-prescrving interpolation,
Mon. Weo,therRe,u..117, 102-709,1989
Acknowledgments. \!-e thank thrcc arronvrÌousÌc-
vierversfor their constnrctivccorrrrnents.TÌris researcÌrÌras
C.Nobre and L Trosnikov, Center for W-eathcr Forecast
dv CNPq (Brrrzil).
l ) c c r sr p o n s o r c b
and Climate Studies, NationaÌ Institute for Spacc Research
- CPTEC/INPE, Roclovia Presidcnte Dutra, krn 40 - SP,
References CEP 12630-000, Cachoeira Paulista, SP, Brazil (e-mail:
br)
igor@cptcc.inpe.
Artaxo, P., E. T. Fcrnandcs, ,J. V. \Iartins, Ì\{. A. Yama-
soe, K. Ì\'1.Longo, P. V. Hobbs, and W. N'Íaenhaut,Large
scale clernental composition of acrosols rncasured during (Received
September 9, 1997;revisedApril 3, 1998;
SCAR-B, in SCAR-B Proc'cerlings: Colle'ction of Po,pers April 7, 1998.)
accepted