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Extreme Mechanics Letters 15 (2017) 44–50

Contents lists available at ScienceDirect

Extreme Mechanics Letters


journal homepage: www.elsevier.com/locate/eml

Optimization of compound serpentine–spiral structure for


ultra-stretchable electronics
Mutee U. Rehman, Jhonathan P. Rojas *
Electrical Engineering Department, King Fahd University of Petroleum and Minerals (KFUPM), Dhahran 31261, Saudi Arabia

article info a b s t r a c t
Article history: Stretchable electronics is a rising technology, promising to replace the conventional, brittle and rigid
Received 27 January 2017 electronics for applications that demand mechanical compliance to irregular, complex and mobile shapes.
Received in revised form 4 April 2017 Several approaches have been proposed to find an optimum balance between electrical and mechanical
Accepted 22 May 2017
characteristics. These include finding new flexible electronic materials, integrating both organic and
Available online 30 May 2017
inorganic materials or incorporating structural modifications to conventional materials, thus achieving
flexibility and stretchability. Previously, the use of spiral-based structures made entirely out of silicon,
Keywords:
Stretchable electronics a well-mature and high-performing material, has been proposed as a platform for ultra-stretchable
Flexible electronics electronic applications. In this paper we have demonstrated the use of spiral-based compound, fractal-
Serpentine structure inspired structures to optimize and greatly reduce the stress and strain distribution along them. The
Spiral structure integration of double-arm spirals with variants of serpentine and horseshoe structures has been con-
Finite element analysis sidered and their mechanical response to an applied deformation has been performed through finite
element analysis (FEA). The proposed compound structures provide outstanding stretching capabilities
and demonstrate up to ∼55% reduction in stress/strain, as well as a more uniform distribution as com-
pared to the original, un-optimized spiral-based structure. These results show the remarkable potential of
combining structures to optimize their mechanical behavior, thus accomplishing more robust platforms
that will leverage the development of stretchable electronics.
© 2017 Elsevier Ltd. All rights reserved.

1. Introduction stretch or flex. This makes conventional electronics inherently in-


compatible with all these applications where mechanical compli-
With the continuous advancement of electronic systems, new ance is not only useful but essential. Research work is underway to
potential and innovative areas of engineering have emerged to overcome such challenges, finding innovative ways to achieve both
cover an exciting range of novel applications from bio-integrated high electrical and mechanical performance. A number of ground-
devices and wearable technologies to smart cybernetics and soft- breaking ideas have been proposed, where two main approaches
robotics, or self-powered sensor networks as enablers of the can be identified; (I) the use of unconventional materials with
Internet-of-Everything (IoE) and Internet-of-Things (IoT) [1–8]. conventional electric designs, or (II) use of novel strategies and
Along with this surge of application areas, electronic systems are structures to adapt conventional electronics with new mechanical
characteristics [10,12–15].
being presented with tough challenges in terms of new mechanical
In relation to unconventional materials, organic or polymeric
requirements and demands. For example, bio-integrated devices
materials are the natural choice due to their excellent mechani-
and wearable electronics, which deal with complex, mobile, soft,
cal characteristics, giving birth to the notion of flexible, organic
flexible and stretchable biological systems, demand the devices
electronics, which can provide great flexibility and even stretch-
to be conformal to irregular surfaces and to be able to exhibit
ability, in contrast to conventionally brittle, inorganic-based de-
certain degree of flexibility and stretchability while retaining the vices [10,16–18]. However, their range of applications is, at the
high electrical performance of conventional electronics, thus still moment, limited due to their lower electrical performance, evi-
enabling fast and efficient processing of high amount of informa- dently lower compared to silicon, and inability to handle high tem-
tion [9–11]. Unluckily, conventional electronics, mostly based on perature processing [19,20]. Alternatively, 1D structures, such as
silicon, are rigid and brittle in nature, thus lacking the ability to nanowires or carbon nanotubes, and 2D atomic structures, such as
graphene or transition metal dichalcogenide nanosheets (TMDC),
are still far from achieving the integration level and layout com-
* Corresponding author. plexity of current silicon-based electronics despite their excellent
E-mail addresses: g201404680@kfupm.edu.sa (M.U. Rehman),
jprojas@kfupm.edu.sa (J.P. Rojas). potential electronic properties [20].

http://dx.doi.org/10.1016/j.eml.2017.05.004
2352-4316/© 2017 Elsevier Ltd. All rights reserved.
M.U. Rehman, J.P. Rojas / Extreme Mechanics Letters 15 (2017) 44–50 45

The alternative second approach, on the other hand, exploits the serpentine-based structures with the same in-plane area (plastic
fact that the flexural rigidity of most stiff materials can be dras- deformation reached at ∼100% applied strain with serpentine-
tically reduced by reducing their thickness down to microscopic based structures, compared to 200% for the spiral). In fact, the use
or nanoscopic features, thus becoming flexible and able to bend to of spirals as ultra-stretchable interconnects has been already pro-
even very small radii [21]. For example, silicon, which is brittle and posed by Huang et al. [22] earlier on, where a topology of silicon-
rigid in nature, becomes flexible when its thickness is reduced to based circular islands, meant to host electronics, were physically
micro- or nanoscale, thus enabling devices made on ultra-thin sili- interconnected through silicon spiral springs in a 2D network. In
con sheets to display even high levels of flexibility, while retaining this work, a very large area expansion ratio of 51 times the original
their excellent electric characteristics [10,19,22–26]. Further struc- size was achieved, which can be extremely advantageous in macro-
tural modifications and smart architectures in the thin membranes electronics applications. Expanding on this, it has been demon-
can expand their mechanical characteristics to go beyond flexibil- strated that the stretchability ratio can be even further improved
ity and even reach stretchability. For instance, ultra-thin silicon by increasing the number of the spiral springs in an area-efficient
sheets can be structured to have a wavy profile, stretchable in na- way. Thus, an all silicon-based network with hexagonal islands was
ture, when transferred onto a pre-strained polydimethylsiloxane proposed, where the islands were physically interconnected with
(PDMS) sheet. This wavy shape in the structure provides end to end double-arm spiral structures, such as the one shown in Fig. 1(a),
stretchability and offers elastic response when strain is applied to reaching an unprecedented stretch ratio of more than 1000%. Ad-
the structure [10,15,27–30]. A similar strategy is applied by replac- ditionally, the base of spring arms were modified with serpentine-
ing the straight silicon sheets with serpentine traces. In this case like structures to mitigate the effect of high strain at both ends,
the level of stretchability can be carefully designed and improved, thus reducing the localized strain at these points by half and
because higher elongation can be reached by the buckling-induced, evenly distributing it throughout the spiral structure [19]. Practical
twisting deformation and sequential unfolding of the serpentine implementations that use spiral structures to build highly stretch-
structures [31]. An immediate extension to these strategies consist able systems for diverse applications have been demonstrated
in arranging the brittle semiconducting materials, containing the as well. For instance, Mamidanna et al. [43] demonstrated the
active electronics, in arrays of rigid islands, which are spatially excellent mechanic and electric performance of spiral-shaped, re-
distributed over an elastic substrate and electrically joined through active ink-based interconnects, showing outstanding stretchability
especially designed metallic interconnects [32–37]. The design of (160%–180%) with only ∼2.5% variation in electrical resistance
these interconnects is prepared in a way to mitigate the strain after being subjected to 1000 elongation cycles. More recently,
induced during the flexing, stretching, or even twisting. The main a spiral-inspired stretchable thermoelectric generator (TEG) was
idea behind this arrangement is to minimize the stress localization shown to, interestingly, generate higher electric power while being
at the brittle region of the electronics [13]. Another benefit of this stretched. This can be easily explained since the temperature gra-
scheme is that it provides the freedom to separate and reorganize
dient increases at stretching, given the adequate conditions [44].
the different components of the system, such as power manage-
Inspired by these all-silicon, spiral-based structures and by
ment, sensing modules, communication, etc.
the concept of fractals, this letter studies, through finite element
Unlike the islands, interconnects can be stretched due to their
analysis (FEA), the effect of replacing the spiral’s arms with ser-
structure. Designing interconnects into stretchable forms can re-
pentine and horseshoe structures for maximum stress and strain
sult in structures that can withstand large strain deformations. Kim
reduction, while maintaining an efficient use of area. This fractal
et al. [38] developed a concept to build a network of islands on
inspired concept, although not self-repeating, consists of the effec-
an elastomer and then connecting the islands through buckled-
tive, combined use of spiral, serpentine and horseshoe structures
arch shaped interconnects. Upon the application of applied strain,
(a structure within a structure). The simulation results showed
interconnects move out of the plane to mitigate the effect of
a considerable reduction in stress and strain, up to 42%, for the
the applied pressure. In the same work, an alternative structure
compound serpentine–spiral structure compared with the original
was also proposed by replacing the straight-arch-shaped, buckled
spiral. Moreover, even further reduction was achieved, up to ∼55%
interconnects with effectively longer serpentine bridges such that
compared with the original spiral, through the optimized com-
the effect of external strain is compensated by the change in height
pound serpentine–spiral with horseshoe structures at the arms’
and geometry of non-coplanar serpentines. A powerful alternative
configuration comes from naturally occurring structures known as start and end.
fractals, a self-repeating structure that can provide stretchability to
a larger extent. The use of fractal structures, such as Peano, Greek 2. Finite element analysis
cross or Vicsek, for stretchable electronics was demonstrated by
Fan et al. [39] in a health monitoring and communication appli- In general, serpentine/horseshoe structures contain periodic
cation. It also showed that higher order fractal structures demon- cells; one unit cell with equal halves with each unit cell containing
strate better stretchability; for example, third order Peano layout two half circles of radius R, thickness t, arch angle α , width w, S
showed more than 20% stretchability which is even higher than is the end-to-end distance and length l between the half circles
skin’s elastic limit. Recently, Yan et al. [40] developed a novel (reference schematic can be seen at the inset of Fig. 3(a)). The
technique to build complex 3D out-of-plane topologies using mul- analytical solution of the in-plane serpentine/horseshoe mechanic
tilayer 2D precursors on a pre-strained substrate, studying the use behavior has been studied in detail in previous works [45–47].
of a variety of geometries, such as circular cages, blooming flower, The general equation for end-to-end distance, S, in case of
entangled wavy arcs, etc., with the potential for innovative out-of- horseshoe serpentine structure, presented in [45], is given as,
plane, stretchable applications, like a demonstrated spiral-based
( )
l
tunable inductor for wireless communication. Similarly by using S = 4 R cos α − sin α . (1)
2
compressive buckling Xu et al. [41] demonstrated to transform
2D structures into 3D. Several 3D geometries were studied that The above equation shows that for higher stretchability, the radius
resulted from their 2D precursors like Helix, toroids and spirals. R of the half-circle plays a vital role and is directly proportional
The use of spiral structures is of especial interest for us due to the end-to-end displacement, whereas the thickness t of the
to their advantageous mechanical characteristics. For instance, structure will have no effect.
it has been recently demonstrated by Lv et al. [42] that spiral- Additionally, a useful non-linear theoretical model for fractal-
based structures can provide larger stretchability as compared to inspired horseshoe microstructures has been already developed
46 M.U. Rehman, J.P. Rojas / Extreme Mechanics Letters 15 (2017) 44–50

Fig. 1. Spiral Structures with triangular ends. (a) Schematic of a fully stretched
spiral structure with two arms and triangular ends. (b) Stress comparison between
the spiral with and without triangular ends along the arms. (c) Strain distribution
comparison between the spiral with and without triangular ends along the arms. Fig. 2. Spiral structure with serpentine arms. Schematics of (a) serpentine structure
with unequal circular halves, and (b) serpentine structure of equal circular halves.
(c) Stress comparison between two serpentine/spiral structures along the arms. (d)
Strain distribution comparison between two serpentine structures along the arms.
by Ma et al. [48], which also demonstrated that by increasing the
order of the horseshoe, the stretchability of the system would be
improved. In our case, we are interested in the incorporation of
serpentine structures, with α = l = 0, within the spiral design in mind area and fabrication constrains. In the case of the spiral,
in order to have a simpler design with less area usage. Later on, we chose a width of 5 µm and the radius of 250 µm, such that the
we also incorporated horseshoe structures to minimize stress and strain reaches to a maximum of 1%. For the case of the serpentine
strain in specific areas only. Although horseshoe structures might the width remains the same (5 µm) and the radius R of each half-
circle was selected to be 14.5 µm, mainly considering an adequate
provide better stretchability and less stress localization, we used
spacing between the spiral’s inner circle (250 µm) and serpentine’s
them partially in our structure mainly because they take up more
half-circle (trough of the serpentine). In addition, the maximum
space than a simple serpentine, especially if we consider the use
stretchability achievable using the spiral structure with two arms
of several turns around the spiral to maximize the stretch ratio,
is dependent on the number of turns in the spiral. This is shown by
without utilizing too much area.
the equation below.
The maximum strain in the case of the spiral structure is given
as [19]: Emax = 2π N (4)
w
εmax = (2) where Emax and N represent the maximum stretchability achiev-
2RS − w able and number of turns of the arms respectively. Eq. (4) is a
where RS is the radius of the inner circle of the spiral (Fig. 1(a)), simplified expression, which shows us that the main parameter for
and w is the width of the arms. Similarly, the maximum strain in reaching a specific stretchability is simply the number of turns N.
the case of the serpentine with α = l = 0, can be express as [45]: We studied several variants of the serpentine/horseshoe struc-
6w tures and their mechanical response was analyzed through finite
εmax = (3) element simulations. At first, by replacing the spiral’s arms with
R−w serpentines the stress and strain distribution was analyzed to iden-
where R is the radius of the inner half-circle in the serpentine, and tify weak areas. Subsequently, the arms’ structure was further opti-
w is the width of the arm (Fig. 2(b)). mized, where the main objective was to not only reduce the strain
Both the above Eqs. (2) and (3) show that the maximum strain but also to minimize the stress localization near the critical areas;
is directly proportional to the width and inversely proportional to the starting and the ending of spiral’s arms. Finally, optimized
the radius of the half-circle. Consequently, the design should try serpentine–spiral structures were analyzed and their performance
to maximize the radius to width ratio of both structures, bearing was compared with the original spiral-based structure. To carry
M.U. Rehman, J.P. Rojas / Extreme Mechanics Letters 15 (2017) 44–50 47

out the finite element simulations COMSOL Multiphysics was used.


2D geometries, designed in SOLIDWORKS, were imported into
COMSOL Multiphysics using its CAD import tool and then extruded
to 3D at a height of 50 µm (thickness of thin-silicon substrate).
The geometry was partitioned into different domains for better
mesh distribution efficiency. The top surface of the inner circle was
used to create a coarse quad-based mesh, while the arms were
used to create finer triangular-based mesh for highest detail. Using
the sweep function, the top layer meshes were propagated to the
whole geometry. For boundary conditions, one arm was kept fixed
while the other was subjected to a prescribed displacement, as
shown in Fig. 1(a), and the stress and strain values were analyzed
at a maximum displacement of 1.8 mm, reached in gradual steps of
50 µm. We also included the effect of geometric non-linearity due
to the large deformation of the structure. Finally, silicon (single-
crystal isotropic) was used from the material library, although an
important point to clarify is that silicon has an anisotropic nature,
and its electrical and mechanical properties will depend on its crys-
tal orientation. In fact, a variation as big as 45% may be observed
in the elastic modulus of silicon depending upon its orientation.
In our particular case, we chose to work with a standard (100)
Si wafer, in which the X - and Y -axes (⟨110⟩ direction; parallel
and perpendicular to (100) wafer’s flat), will both have an elastic
modulus of 169 GPa (value used in our simulations). If a different
orientation should be used, then it should be considered that the
smallest elastic modulus will be found in the ⟨100⟩ direction (130
GPa), whereas the maximum modulus value will be in the ⟨111⟩
direction (188 GPa) [49].

3. Results and discussion

As mentioned earlier, this research work studies several vari-


ants of serpentine structures and their combination with the spi-
ral structure to demonstrate their effectiveness for stretchable
electronics. The performance of these optimized structures was
compared with the original spiral structure presented in Fig. 1(a). Fig. 3. Spiral structure with equal serpentine halves and horseshoes at the
Therefore, we first simulated the original spiral structure with end/beginning of arms. Schematics of (a) serpentine/spiral structure with horseshoe
at the end (Inset shows the main parameters of a horseshoe structure), and (b)
two arms and later we added triangular-like end structures at the with horseshoe at the start. (c) Stress comparison along the arms, and (d) strain
extremes of each arm. This was done to minimize and redistribute distribution comparison along the arms.
the stress localized at those end points and to represent more
accurately the actual case where there should be a smoother area
transition between the islands and the arms of the spirals (inset of important role in the performance of the structure. To study the
Fig. 1(a)). Additionally, Fig. 1(a) shows the fully extended original effect of radius, we compared two versions of serpentine. The
spiral with triangular ends where one arm is fixed and the other version shown in Fig. 2(a) is a serpentine structure with each
is subjected to the displacement, while Fig. 1(b) and (c) show the circular half having different radius represented by R1 and R2 ,
comparison between the stress and strain distribution along the with the values of 14.5 µm and 9.5 µm respectively In this case
arms for both structures. The two strains in the graph represent the trough is bigger (represented by R1 ) in size as compared to
the compression and elongation in each side of the arm, the upper the crest (represented by R2 ). The other version has both circular
and the lower side, while the two halves represent the strain in halves of the serpentine with equal radius R, where R = R1 , the
each arm, left and right. The points with the maximum stress and longest radius, as shown in Fig. 2(b). The comparison of stress
strain, in the case of the spiral structure without triangular ends, and strain between the two structures is shown in Fig. 2(c) and
were expectedly at the extreme ends of the spiral’s arms. This (d) respectively. Simulation results show that the structure with
maximum stress and strain were 8698 MPa and 4.23% respectively, equal radius halves resulted in lower stress/strain as compared
as a result of a prescribed displacement of 1.8 mm (∼250% applied to the structure with different halves (very similar results were
deformation). By the addition of transitional triangular structures obtained for the case where the trough was smaller than the crest
at both ends of the spiral’s arms, the peak stress and strain values as presented in the supplementary material). The maximum stress
were reduced to 4284 MPa and 1.49% respectively (these values in case of unequal halves was found to be at the start of the spiral’s
will be our reference from now on). Since these end points are to arm under displacement with a value of 2309 MPa which is 46%
be connected between islands, it is vital to lower the stress/strain less than the original spiral in Fig. 1(a), while the maximum peak
at these weak localizations. Interestingly, the addition of triangular strain was found to be 0.93% at the start of the triangular base
ends shifted the maximum stress/strain to the start of the spiral’s structure in the arm under displacement, which is 37.6% less than
arms, as shown in Fig. 1(b) and (c). the original spiral. On the other hand, the structure with equal
The next step after analyzing the spiral structure and noting radius halves showed a reduced peak stress and strain, at the start
its maximum stress localization points, was to replace the spiral’s of the spiral’s arm under displacement, of 2265 MPa and 0.87%
arms with different variants of serpentine structures. As men- respectively, which represents a much higher respective reduction
tioned above, the radius of the arch of the serpentine plays a very of 47.12% and 41% less than the original spiral structure.
48 M.U. Rehman, J.P. Rojas / Extreme Mechanics Letters 15 (2017) 44–50

Fig. 4. Structure with equal serpentine halves and horseshoes at the beginning and end of the arms. Schematics of (a) serpentine/spiral structure with two arms and horseshoe
structure, and (b) stretched structure. (c) 3D stress distribution along the arms, and (d) 3D strain distribution along the arms. (e) Stress comparison between original spiral
and compound structure along their arms, and (f) strain distribution comparison between original spiral and compound structure along their arms.

Since it has been observed from the initial simulations that Finally, we have combined both modifications presented in
the maximum points for stress and strain points are either at the Fig. 3(a) and (b) into a single, optimized structure and compared its
beginning or at the end of the spiral’s structure, therefore we performance with the original un-optimized spiral, from Fig. 1(a).
have focused our further optimization steps on those points, to The resultant structure has serpentines with equal radius and
reduce and redistribute the stress localization. In order to improve horseshoe structures at both start and end of the spiral’s arms, as
these weaker regions, we have added horseshoe structures at the shown in Fig. 4(a), and in Fig. 4(b) being fully stretched. Fig. 4(c)
end, shown in Fig. 3(a), and at the beginning of the spiral’s arms, and (d) show the stress and strain distribution along the spiral’s
shown in Fig. 3(b), given that there is more area available at those arms. The simulation results are then compared with the initial
regions. Moreover, the starting point of the spiral’s arms was also results from the spiral structure with triangular ends shown in
optimized to allow the arm to move freely, with higher mobility Fig. 1(b) and (c). These results clearly show the outstanding me-
as an improved transition point from the rigid circular island to chanical performance improvement of the optimized, compound
the serpentine structure (as shown in Fig. 3(b)). Their performance serpentine–spiral structure with horseshoe ends. The maximum
was compared in order to study the effect of each modification values for the stress and strain, due to the incorporated modifi-
separately. From Fig. 3(c), for the case of the structure with horse- cations, were observed to be 1779 MPa and 0.69% along the arms,
shoes at the end of the spiral’s arms, the peak stress was reduced which represents 58.47% and 53.7% less than the original spiral re-
compared to the previous cases, and the maximum value was spectively, as shown in Fig. 4(e) and (f). Likewise, a much smoother
noted to be 2133 MPa, located at the beginning of the fixed arm, distribution is also apparent from the same figures. Based on these
which is 50.2% less than the original spiral in Fig. 1(a). Similarly, simulations it could be inferred that the effective implementation
the maximum value of strain was noted to be 0.82%, which is 45% of compound structures in key locations can greatly help to re-
less than original spiral structure. On the other hand, the structure duce stress and strain and enable a better distribution along the
with horseshoes at the start of the spiral’s arms showed higher structure as compared to the original structure by itself. Moreover,
reduction compared to the one with horseshoes at the end. The by the addition of more turns, the serpentine–spiral structures
peak stress was noted to be at the end of the fixed serpentine stretchability can be increased to many folds depending on the
arm, with values of 1866 MPa, 56.44% less than the original spiral, number of turns added. Finally, addition of horseshoe structures
while the strain was found to be 0.72%, which is also 51.7% less greatly improved the structure’s performance but at the price of
than original spiral structure. This demonstrate the importance of higher use of space. In that sense, we can say that there is a compro-
designing a good transition between the rigid and the stretching mise between stretchability and area efficiency, and finding their
structures. balance can be crucial for any given application.
M.U. Rehman, J.P. Rojas / Extreme Mechanics Letters 15 (2017) 44–50 49

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