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Article history: Integrating multiple utility outputs to obtain better efficient system has been a good option. After cogen-
Received 2 November 2016 eration and trigeneration, polygeneration emerges as a possible sustainable solution with optimum
Received in revised form 15 May 2017 resource utilization, better efficiency and environment friendliness. Several possible polygeneration
Accepted 18 May 2017
has been conceptualized, performance assessed theoretically as available in literature. Both inputs and
outputs vary in these reported works. A few prototype development and experimental result analysis
are also reported. Several optimization tools based on objective function are used to develop efficient
Keywords:
polygeneration. Assessment criteria of polygeneration are also multi dimensional and may be defined
Polygeneration
Sustainable energy
on a case to case basis with definite objective. In this paper a comprehensive review of available literature
Energy system design is done to assess the status of polygeneration as a possible sustainable energy solution. Possible future
Performance assessment research in this field is also logically predicted at the end of this review.
Sustainability Ó 2017 Elsevier Ltd. All rights reserved.
Contents
1. Introduction . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . 89
2. Fuel inputs to polygeneration . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . 92
2.1. Coal based polygeneration . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . 93
2.2. Biomass based and biomass hybrid polygeneration . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . 93
2.3. Solar based and solar hybrid polygeneration . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . 94
3. Energy conversion devices for power/electricity . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . 95
4. Outputs of polygeneration . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . 97
5. Scale/capacity of polygeneration . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . 100
6. Analysis and assessment of polygeneration . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . 101
7. CO2 capture in polygeneration . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . 104
8. Optimization of polygeneration. . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . 104
9. Operation and control of polygeneration . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . 104
10. Sustainability issues . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . 106
⇑ Corresponding author.
E-mail addresses: de_sudipta@rediffmail.com, sde@mech.jdvu.ac.in (S. De).
1
Present affiliation: Centre for Energy, Indian Institute of Technology Guwahati, Guwahati 781039, India.
http://dx.doi.org/10.1016/j.apenergy.2017.05.129
0306-2619/Ó 2017 Elsevier Ltd. All rights reserved.
K. Jana et al. / Applied Energy 202 (2017) 88–111 89
(a)
Fuel Power Plant Electricity
Effluent
(b)
Effluent
(c)
Electricity
Effluent
Heat, Power
(d)
Electricity
Ulity heat
Polygeneraon Plant
Resources Refrigeraon
Coal
Biomass Chemicals etc.
Solar
Wind etc. Effluent
Fig. 1. (a) Power generation, (b) cogeneration, (c) trigeneration and (d) polygeneration.
Studies on
polygeneraon
Table 1
Summary of polygeneration design and simulation.
Author Input energy sources Outputs Energy conversion devices for Objectives
power/electricity
Gao et al. [18] Natural gas Power, methanol CCGT System design
De Kam et al. [19] Biomass Ethanol, power, heat Steam turbine Aspen PlusÒ simulation
Rubio-Maya et al. [11] Natural gas, solar energy Electricity, heating, cooling fresh Gas turbine, fuel cell, Stirling Design optimization
water engine
Kyriakarakos et al. Wind energy, solar energy Electricity, water, H2 Wind turbine, fuel cell Simulation and optimization
[20]
Pellegrini and Oliveira Sugarcane Sugar, ethanol, electricity Steam turbine Exergy optimization
Jr. [21]
Li et al. [22] Coal, coke oven gas Methanol, dimethyl ether, – Simulation and exergoeconomic
dimethyl carbonate analysis
Chen et al. [23] Coal, biomass Power, liquid fuels, chemicals – Optimization of process design
Ilic et al. [24] Biomass, molasses Ethanol, biogas, electricity, heat – Optimization
Ahmadi et al. [25] – Power, cooling, heating CCGT Multi-objective optimization
Maraver et al. [26] – Power, cooling, desalinated water Organic rankine cycle Simulation and performance
assessment
Calise et al. [27] Vegetable oil, solar thermal Electricity, space heating, cooling Reciprocating engine Dynamic simulation (by TRNsys)
domestic hot water
Calise et al. [28] Hybrid solar photovoltaic/ Electricity, space heating, cooling PV Dynamic simulation (by TRNsysÒ)
thermal collectors (PVT) domestic hot water
Samavati et al. [29] Syngas and hydrogen Electricity and heating Solid oxide fuel cell Design and simulation
Song et al. [30] Biomass Ethanol, power, heat Steam turbine Influence of drying process
Yi et al. [31] Coke-oven gas and coal gasified Electricity, methanol, DME CCGT Aspen PlusÒ simulation and
gas optimization
Li et al. [32] Coal Methanol, power CCGT Aspen PlusÒ simulation
Lythcke-Jørgensen Biomass Power, heat, ethanol Steam turbine Exergy analysis
et al. [33]
Salkuyeh and Adams II Coal Power, methanol, DME Gas turbine, steam turbine Chemical looping
[34]
Narvaez et al. [35] Syngas Power, methanol CCGT Process design for small and
medium scale
Zhang et al. [36] Coal Electricity, methanol CCGT Optimal design (MINLP)
Li et al. [37] Coal Natural gas, power CCGT Exergy analysis
Buonomano et al. [38] Solar energy Heating, cooling, electricity PV Design, simulation and thermo-
economic optimization
Calise et al. [39] Solar PV/T, biomass Power, heating, cooling, fresh PV Exergy analysis
water
Salkuyeh and Adams II Shale gas Power, ethylene CCGT Process design (Aspen PlusÒ
[40] simulation)
Bose et al. [41] Coal Power, urea, utility heat CCGT Process design (Aspen PlusÒ
simulation)
Jana and De [42] Agricultural waste Power, heat, chill, ethanol CCGT Process design (Aspen PlusÒ
simulation)
Jana and De [43] Coconut fiber Power, desalinated water, heat, CCGT Process design (Aspen PlusÒ
chill simulation)
Tock and Marechal Biomass, coal, natural gas H2, electricity, heat and captured Gas turbine, steam turbine, Multi-objective optimization
[44] CO2 fuel cell
Lythcke-Jørgensen and Biomass (straw) Power, heat, ethanol Steam turbine Design optimization
Haglind [45]
Hao et al. [46] Coal and coke oven gas Dimethyl ether, methanol and CCGT System modeling
electricity
Yu and Chien [47] Coal SNG, ammonia, electricity Steam turbine Design and economic evaluation
Guo et al. [48] Lignite Electricity, tar CCGT Simulation
Zhu et al. [49] Coal H2, power CCGT Modeling (dual chemical looping
process)
Farhat and Coal H2, power, urea, ammonia CCGT Economic modeling
Reichelstein [50]
Calise et al. [51] Solar PV/T Electricity, space heating, chilling, PV Dynamic simulation and
hot water thermoeconomic optimization
Kieffer et al. [52] Natural gas, municipal solid Electricity, transportation fuel CCGT Techno-economic modeling
waste (FT)
Mohan et al. [53] Solar thermal Chill, clean water, domestic hot – Dynamic simulation (by TRNsys)
water and economic modeling
Rahman and – Electricity, heating, distilled Modeling and dynamic simulation
Malmquist [54] water
Soutullo et al. [55] Solar thermal, PV, PEM fuel cell, Heating, cooling, electricity PV, PEM fuel cell TRNsys simulation and performance
biomass assessment
A few experimental and pilot plants of polygeneration are also water [57]. The plant was based on compression ignition engine
considered in a few studies. Design and experimental investigation of 9.9 kW power and it was run by plant oil. Paleta et al. designed
of a pilot plant of polygeneration (190 kW biomass fixed bed gasi- and tested a polygeneration energy container for remote commu-
fier) was reported by Ma et al. [56]. Hossain et al. developed a poly- nities to test design issues and solve operation and maintenance
generation for electricity, food preparation, cold storage and pure challenges associated with autonomous electricity production sys-
92 K. Jana et al. / Applied Energy 202 (2017) 88–111
Table 2
Brief energy scenario of the different countries in the world.
Continent Country Total energy consumption (Mtoe) Total electricity consumption (Mtoe) Percentage of renewable electricity (%)
Asia India 882 88.3 14.1
China 3101 423.1 24.7
Europe United Kingdom 179 27 26.3
Norway 32 2.7 97.9
America United States 2196 110 13.8
Australia Australia 126 19 15.2
Africa Egypt 80 12.5 8.9
South Africa 138 17.8 3.3
Table 3
Regional estimation of fossil fuel reserves in India.
Arunachal Pradesh, Uttarakhand, etc. Bio energy is abundant in based polygeneration with power generation and urea production
most of the states as India is an agro based country. Thus India is is shown in Fig. 5. In this polygeneration process, coal is used
rich in renewable resources varying at different locations [72]. To through gasification. CO2 is captured in this system and utilized
set up useful polygeneration with renewable energy integration for urea production through system integration.
of these locally available resources are critical. As a whole, India
has potential development of both renewable and coal based
polygeneration. 2.2. Biomass based and biomass hybrid polygeneration
food crops (sugar, corn, rape seed, etc.) were used to produce bio- using rice straw as cattle fodder only. There are several challenges
ethanol or bio-diesel [87]. In second generation biofuel production on technology development to utilize this waste as energy
process, wood, crop waste, organic waste, etc are used for biofuel resources [77]. To utilize this waste, decentralized technology
production. Hence, there is no constraint related to food security. development is more suitable [96]. However, centralized concen-
Yield of biofuel is increased in third generation of biofuel produc- tration of these may happen for agro-industrial wastes say, sugar-
tion [88]. Carbon capture and storage can be integrated with vari- cane bagasse. Developing technology for using agricultural waste
ous biofuel production processes to obtain a net negative system as energy resources matching with local availability and secondary
that may be called fourth generation biofuel production [89]. energy needs may be very useful for future sustainable solution,
One of the greatest sources of biomass is agricultural waste specifically for rural areas [57]. In Table 4, summary of papers on
without affecting food security [90]. Agricultural waste is produced biomass based polygeneration is compiled. In this table different
in agro-processes and many of these have good potential to be kind of biomass inputs, their conversion process and outputs of
energy resources [91,92]. Thermochemical properties of these polygeneration are given. From this table it is noted that wide
waste widely vary with the type of crop [93]. Depending on these range of biomass can be used as input energy sources in polygen-
properties, potential of biomass for power generation or biofuels eration and through these polygeneration bio-fuel (methanol,
production are also different. Typical feature of an agricultural ethanol, DME, etc.) is an important output [108–110].
waste is its availability confined within rural areas. Hence, logistics
of biomass supply is important [94]Generation of the waste over 2.3. Solar based and solar hybrid polygeneration
the year also varies widely [95]. For seasonal crops (say, rice) waste
are generated in bulk during reaping of the crops. A few food pro- Solar energy is a form of renewable energy available almost all
cessing industries also produce waste (say, sugarcane bagasse) over the world with different intensity. The countries dependent
from agricultural crops. These waste are available in concentrated on the conventional energy sources should adopt policies for
manner. For plantation crops (say, coconut), waste may be avail- enhancing the solar energy market [111]. It can be utilized as an
able more or less at a uniform rate over the year. Use of a particular energy source of polygeneration. However, polygeneration is very
agricultural waste also varies widely depending on its type, its difficult to be achieved by only solar energy input due to low
available amount and geographical location of availability and energy concentration [27]. In majority of the cases, the solar
existing practice of the local people due to various socio- energy is hybridized with the other forms of renewable energy like
economic reasons. These agricultural waste have sufficient calorific the biomass energy and the fuel cells to produce utility outputs as
values. Hence, it can be utilized for better value-added processes obtained from the literature and shown in Fig. 8. The major renew-
with developed technology [93]. For example, rice straw may be able energy sources hybridized with solar thermal or photovoltaic
used for heating, electricity generation or ethanol production collectors are biomass gasifier and fuel cells [112] as given in
either through thermochemical or biochemical route. Economic Table 5. As noted from this table, solar thermal collectors have
value of this utilization will be better than existing practice of more applications than solar photovoltaic collectors in polygener-
K. Jana et al. / Applied Energy 202 (2017) 88–111 95
Particulate
removal CO shift
CO2
removal
H2 rich
Water Methanation
quenching Syngas Syngas
compression
Process &
steam Ammonia
CO2 synthesis
Cryogenic (N2+3H2↔2NH3)
purification
Coal stock Coal mill Gasifier
N2 wash
Compressor
N2
ASU NH3
Combustor
Air Compressor
Flue
Gas gas
HRSG
turbine
Steam
Turbine
Pump
Steam
turbine
Condenser Pump
Condenser
Heat
Process heat
ation systems. The fuels cell hybridized polygeneration generally 3. Energy conversion devices for power/electricity
produces electricity with cooling, heating and potable water as
the utilities. Biomass hybridized polygeneration system generally Power is generally a major output of polygeneration. Hence,
yields biofuels like ethanol, methanol, etc with the electricity, prime movers or energy conversion devices are required for power
heating and cooling as the outputs. Hybrid polygeneration helps generation in a polygeneration. These are selected according to
to reduce the energy storage capacity and it has the potential to input fuels, capacity, economy, availability, etc [129]. In Fig. 9, var-
utilize multiple intermittent energy resources efficiently [128]. ious types of prime movers of polygeneration are shown. Cost-
96 K. Jana et al. / Applied Energy 202 (2017) 88–111
To ethanol
producon
LPST
unit
Syngas Syngas
Splier compressor
cooler
Catalyst
Combuson Superheater-
GT Reheater
chamber
Gasifier
Air
Rice Ai compressor Make-up Pump
straw water Economizer-
Air Evaporator
Condenser
Ash
Waste heat
recovery
HPST
To vapor
absorpon Process To stack
chiller heater
Fig. 6. Schematic of polygeneration process for power, ethanol, heat and chill [64].
B36
Q
S56
Q-PRO2 B37
S60
S59
B1 B2
PRO-IN PRO-OUT S20
B35 S64
S55
B38
S63
S4
S50
S62 B32
S54
H2O-ETOH
B31
S21 B34
S53 Hydrous
CO2-FREE ethanol
ETH-SYNT
S61
COL-GAS H2O
B27
MEA-based acid gas removal process
WGS
B29 CO2
S48
S52 H2-CO
B25
CO2-CAPT
Syngas
benefit analyses of polygeneration play an important role in prime toming cycle to increase the overall thermodynamic efficiency
mover selection. Gas turbine is used to generate power for gaseous [43]. Micro-gas turbine is selected as prime movers for small scale
fuels (say, natural gas or syngas derived through gasification. But and standalone polygeneration [54]. Steam turbine is useful for
impurities in the syngas should be within the permissible limit direct combustion of solid fuel (coal/biomass combustion). Where
[130]. In combined cycle gas turbine (CCGT), gas turbine cycle is available heat is at relatively low temperature (say geothermal
used as topping cycle and steam turbine cycle may be used as bot- heat, solar thermal heat), organic Rankine cycle (ORC) is suitable
K. Jana et al. / Applied Energy 202 (2017) 88–111 97
Table 4
Summary of biomass based and biomass hybrid polygeneration.
Output utilities
Hybridized
Electricity
Fuel cell
Cooling
Biomass
gasifier/digester
Heating and
Solar drying
PV/ Wind
Thermal
Biofuels
Micro gas
turbine
Hydrogen
Geothermal
Oxygen
Fig. 8. Possible hybridization and output utilities of solar thermal/photovoltaic based polygeneration.
[26]. For ORC, selection of working fluid is crucial [131]. Supercrit- 4. Outputs of polygeneration
ical and transcritical CO2 cycle is another option for low tempera-
ture heat recovery and power generation. In Fig. 10, schematics of Polygeneration is designed to deliver multiple utilities. From lit-
gas turbine cycle, Rankine cycle, combined cycle gas turbine eratures, it is observed that polygeneration can deliver different
(CCGT) are shown. For distributed generation, internal combustion types of outputs e.g., energy services, materials, drinking water
engine is preferred due to its low initial cost and robustness [57]. [6,13]. Possible utilities as reported in literature are shown in
As efficiency of fuel cell is high, it has potential to be used for elec- Fig. 11 However, these output utilities are selected according to
tricity generation, though novel material is required and it is highly inputs and utility demands. For decentralized polygeneration, out-
sensitive to impurities [28,29,132]. In this case input fuels should puts should be in line with local demand to cater to local needs.
have high level of purity. Transportation or transmission of utility outputs for long distance
98 K. Jana et al. / Applied Energy 202 (2017) 88–111
Table 5
Solar hybridized polygeneration system.
Fuel
(a) Combustion
chamber
(b)
Steam generator
LPST HPST
Pump
Condenser
Fuel
(c)
Combustion
chamber
LPST HPST
Condenser
Fig. 10. Schematic of (a) gas turbine cycle, (b) Rankine cycle, and (c) combined cycle gas turbine.
(MSF), multi-effect distillation (MED) are examples of heat driven generation during load fluctuation i.e., when electricity demand is
process and reverse osmosis (RO) is an example of power driven less, it can be used for water production and stored for future.
process. When waste heat is available, heat driven desalination is Hence, polygeneration helps to manage the fluctuating-load. Detail
preferred [140]. Power driven water purification is utilized in poly- about control and monitoring is discussed later. Thus, through the
100 K. Jana et al. / Applied Energy 202 (2017) 88–111
multi-generation system water can be produced efficiently and However, outputs must give a reasonable thermodynamic perfor-
economically [141]. mance so that economic performance can be feasible in the long
Hence, outputs of the polygeneration may be selected either run.
according to inputs and configuration or according to local needs.
5. Scale/capacity of polygeneration
To Stack
Syngas compressor
Heat recovery unit
Cyclone
Gasifier
Char
Biomass
Syngas
Process Air Ash Gas
scrubbing Gas cooler
water
Flue gas
E E R S S Gas turbine
Combustor
C V H P P
O A H H
1 2
Process
steam
Pump Air
LPST
Waste heat
Q
R-Q-COND
R-COMSEP
R-FLSH
R-GEN S9
R-COND
S8 S13
S14
S7
R-VALVE2
R-HX S11 S15
R-VALVE1
S12
S10
S6
S16
Q
R-MIX R-Q-EVAP
R-EVAP
R-PUMP
S17
Q
S18
R-FEED
R-Q-ABS
S2
R-ABS
Assessment
Thermodynamics
Techno-economic Socio-economic Environmental Mul-dimensional
(1st law, 2nd law)
Table 6
Summary of assessment methodologies of polygeneration.
Table 7
Summary of polygeneration with CO2 capture and recovery.
efficiency was calculated for cogeneration cycle to find the effects improvement is identified [43]. Two thermodynamic objective
of cycle coupling-configuration on energy cascade utilization functions during the design of polygeneration is to increase energy
[145]. Jing et al. studied the performance of cascade utilization of efficiency and exergy efficiency. Definitions of these two are given
new power generating technologies [146]. Kanoglu and Dincer in following equations:
(2009) assessed cogeneration plant by using energy and exergy
efficiencies [147]. Energy and exergy efficiencies were used to energy equiv alent of utility outputs
energetic efficiency ¼
assess and optimize the co-production of hydrogen and electricity fuel energy input þ other from of energy input
[148]. A few exergy based analysis of polygeneration are also avail- ð1Þ
able in literature [121,149–151]. Apart from first law efficiency and
second law efficiency, some environmental and economic parame- exergetic efficiency ðenergy utilization effciencyÞ
ters were also studied for trigeneration system [152–154].
exergy of output utilities
Similar to power generation, cogeneration and trigeneration, ¼ ð2Þ
thermodynamic analysis is done for polygeneration by 1st and exergy of input utilities
2nd law of thermodynamics. 1st law includes the quantity of However, other thermodynamic parameters like fuel energy
energy but does not include the quality [155]. 2nd law of thermo- savings ratio (FESR), primary energy savings (PES), artificial ther-
dynamics includes both quantity and quality of energy through the mal efficiency, etc are used for polygeneration [26,69].
term of ‘exergy’ 158]. In 2nd law analysis, exergy destructions To be a sustainable energy solution, polygeneration should be
within the polygeneration process are shown and possibility of economically feasible and beneficial. Hence, economic feasibility
K. Jana et al. / Applied Energy 202 (2017) 88–111 103
(a)
Electricity
Utility heat
Polygeneration Unit
Resources Refrigeration
Coal
Biomass H2 etc.
Solid waste
Effluent
Heat, Power
CO2 capture CO2 sequestration
Unit
(b)
Electricity
Utility heat
Polygeneration Unit
Resources Refrigeration
Coal
Biomass H2 etc.
Solid waste
Effluent
Flue gas/syngas
Fig. 17. (a) Polygeneration plant with CO2 capture and (b) polygeneration plant with CO2 capture and utilization.
and viability are tested through techno-economic analysis [156]. As discussed earlier, ‘environment’ is another pillar for
Then, it is analysed through socio-economic parameters for instal- sustainability. Several publications are available on environmental
lation and sustainable operation [157]. Also for decentralized assessment of polygenerations as given in Table 7. In some litera-
applications, socio-economic conditions of locality play an impor- tures, environmental assessments are done based on life cycle
tant role in this regard [145]. Several techno-economic studies of environmental impact including all aspects of environmental
polygeneration are available in literature as given in Table 6 degradation [89,174]. Many authors assessed environmental
though a few papers are available on socio-economic studies of parameters through GHG or CO2 emission [159,175,176]. For
polygeneration. Depending on the demand and economic value polygeneration with carbon capture and storage (CCS) or carbon
of output utilities, ‘usefulness of polygeneration’ may be calculated capture and utilization (CCU), net GHG emission is the main focus-
and compared for different decentralized polygenerations. ing area.
104 K. Jana et al. / Applied Energy 202 (2017) 88–111
Assessment of polygeneration may be done with multi- temperatures, reboiler heat duty can be minimized through poly-
dimensional viewpoint [42,166]. Depending on the objectives of generation. Also, reuse of captured CO2 is possible in the polygen-
polygeneration assessment parameter may be different. These eration. Thus polygeneration is generally efficient than a
parameters can be the objective functions for optimization of poly- standalone unit due to better heat and mass utilization through
generation [166,177]. However, the assessment parameters may be efficient system integration. The life cycle assessment shows that
in combined form, say, exergo-environmental, exergo-economics the polygeneration with CCS facility substantially reduce GHG
or exergo-environmental-economics, etc according to the objective emission [89].
of polygeneration and its evaluation [178]. From the literature
review, it is identified that there is a challenge for developing uni- 8. Optimization of polygeneration
form performance indicator to assess all kinds of polygenerations
on a single platform [12]. Polygeneration is a multi input and multi output system. Poly-
generation is done with single or multiple resources to achieve cost
7. CO2 capture in polygeneration minimization, GHG emission minimization without compromising
the supply of desired quantity of the utilities. Several publications
For coal or biomass based polygeneration, there is a scope of are available on optimization of polygeneration as shown in
CO2 capture as shown in Fig 16. Basic concept of carbon capture Table 8. To design the polygeneration systems the numerical opti-
and utilization are shown in Fig 17. Coal based polygeneration mization techniques are used mainly to proper sizing of the com-
increases CO2 concentration in atmosphere and it leads to climate ponents, judicious use of resources to obtain maximum economic
change. To be a sustainable energy solution, it should be equipped and environmental benefits. Maximum possible combinations are
with CO2 capture and storage (CCS). Energy is consumed in the taken in consideration while designing the polygeneration system.
form of reboiler heat duty and compression power during captur- In the design of a polygeneration system mainly multi objective
ing and storing of CO2. Integration of CCS is done through heat and optimization techniques are used [11,185]. In most of the cases
mass integration in the polygeneration to reduce the overall constrained optimization is used [45]. Mixed Integer Linear pro-
energy penalty. However, captured CO2 may be utilized for produc- gramming is used for the proper sizing of the components of the
tion of value added products to reduce the economic penalty of polygenerations. Some of the objective functions have to be mini-
carbon capture [14,98]. CO2 is also a source of carbon for synthetic mized and some have to be maximized [182]. Non conventional
fuel (methanol, DME) production. Sometimes CO2 is captured after optimization techniques like multi objective evolutionary algo-
water gas shift (WGS) reaction (i.e. pre-combustion capture) to rithm and Particle Swarm Optimization (PSO) yields better results
produce H2 rich syngas or to maintain a desired ratio of CO and in some cases than the conventional optimization algorithms [25].
H2 as given in Table 7. This CO and H2 are used for thermo- In non-conventional techniques often a set of solutions are found
chemical fuel synthesis (methanol, ethanol, DME, etc.) from bio- out. Application of fuzzy logic in the yields better results in the
mass or coal. Available literatures on coal based polygeneration optimization problems.
with CO2 capture and recovery are given in Table 7. The polygener-
ation with CO2 capture is more efficient and cost effective than the 9. Operation and control of polygeneration
stand alone CCS systems. During the process of system integration
of polygeneration, utility heat may be available from various Polygeneration is a multi input and a multi output system.
sources at different temperatures. By utilizing heat at different However, supply of renewable energy is intermittent. Demands
Table 8
Numerical optimization in polygeneration system design.
Table 9
Operation and control of polygeneration process.
of utilities are also different. This supply and demand matching is come from supervisory control and data acquisition (SCADA) sys-
possible through intelligent control during operation as shown in tems [198]. The application of fuzzy logic and petri net analysis
Fig. 18. Literatures available for operation and control of polygen- proves to be better than conventional control systems [192]. In
eration are shown in Table 9. From Table 9 it is concluded that for some cases programmable logic controller (PLC) is also used. In
the proper functioning of a polygeneration plant the synchroniza- recent times advanced numerical computational techniques are
tion of all supply and demand are necessary. In the case of renew- also used. The control system is mainly needed to cater to the vary-
able based polygeneration, the energy sources like solar, wind, etc ing seasonal load with the intermittent renewable energy
are intermittent in nature. The load is also variable in different sea- resources. The PLC proves best suitable controller as the necessary
sons throughout the year. Hence a proper control system is used changes can be made in the control logic by software applications.
for the suitable operation of any polygeneration plant. In polygen- This also minimizes the error [199].
eration systems, mainly the Model Predictive Control is used in The polygeneration systems have several inputs and outputs. So
most of the systems [196]. Some the systems reported in the liter- multi objective optimization is needed to optimize a polygenera-
ature have the application of supervisory control whose inputs tion system. The type and amount of the outputs of a polygenera-
106 K. Jana et al. / Applied Energy 202 (2017) 88–111
tion are mainly decided by the resource availability as well as the the fossil fuel based resources. The fossil fuel reserves are depleting
local demand. Efficient integration of several processes in the same fast and moreover combustion of the fossil fuels have many envi-
system makes it more viable economically and socially. Integration ronmental negativities. So alternatives must be tried to get a sus-
of the various processes like electricity generation, fuel synthesis tainable energy system in the long run. To achieve the
(mostly environmentally benign bio fuels), waste heat recovery, sustainable energy system, two things may be considered (i)
cooling, etc. increases the overall performance of the process. Effi- Increasing the process efficiency to reduce the losses and (ii) fuel
cient control systems are needed for polygenration. Advanced con- switching from fossil fuels to renewable. Polygeneration system
trol mechanisms like SCADA are needed to control the multiple addresses both of these issues where multiple sources are inte-
parameters. In a polygeneration system, the fluctuation of one grated in a proper manner to get multiple utilities. The process
parameter is absorbed in the production of other(s). It makes the integration increases the system efficiency and the uses of the
system even more efficient. The excess heat of solar collectors renewable energy resources reduce the dependence on the deplet-
may be fed to an absorption chiller to produce cooling utility ing reserves of the fossil fuels.
[195]. The objectives of optimization in a polygeneration are also Fig. 19 describes the transition from the fossil fuel based energy
many [195]. The nature inspired algorithms like ant colony opti- systems to renewable based polygeneration. Till now combustion
mization algorithm, differential evolution algorithm, etc are used of fossil fuels is the main source of energy generation in India.
for carrying out multi objective optimization in energy systems The main fossil fuels used in energy generation are coal (electricity
[203]. Researchers have used many efficient algorithms for the generation), oil (transportation sector) and natural gas (power gen-
design of smart energy systems. The multi-period artificial bee col- eration and transportation sector). The two drawbacks of the fossil
ony optimization algorithm is used and its superiority over the fuel based energy systems are limited reserves and the emission of
conventional mixed integer linear programming (MINLP) is shown green house gases along with other effluents which have an envi-
[204]. Moreover, uncertainty is another parameter to be addressed ronmental degradation effect. For these reasons there is a need of
while designing a polygeneration system with the renewable transition from fossil fuel based systems to renewable based sys-
resources. In a polygeneration system, the control and optimiza- tems. Renewable based energy systems emit less environmentally
tion methodologies must be flexible [205]. Thus the advanced con- harmful effluents. But these energy sources are intermittent in nat-
trol strategies like the Model Predictive Control strategy is used to ure. So, proper integration of these available resources at a certain
accommodate all these variations in the best possible way. place can lead to a clean energy system. To make it sustainable
thermodynamic, economic and environmental optimization is
done to form a polygeneration system which has multiple inputs
10. Sustainability issues as well as multiple outputs. The output of a particular process is
the input of another process. The input of the polygeneration
According to the report of the Brundtland commission, ‘‘Sus- system is any renewable energy/hybridized renewable energy/
tainable development is defined as the development that meets hybridized renewable-fossil fuel source and the output utilities
the need of the present without compromising the ability of future are biofuels, hydrogen, potable water, cooling, heating, etc. The
generations to meet their own needs”. So for an energy system to advantages of renewable energy usage are non-depleting reserves
be sustainable it must be economically viable, environmental and low effluent emission. The disadvantage of using renewable
friendly and socially acceptable. Energy plays a pivotal role in the energy is intermittency in nature, high initial cost, etc. Both these
development of a nation. Presently India is mainly dependent on issues are addressed in a polygeneration system. The generation of
Agricultural load
Renewable
Residential load
Fossil Fuels
Industrial Load
Integration of Solar
Heating, cooling
Transportation renewable by
utilities
Load thermodynamic, Biomass
economic,
environmental
Electricity Polygeneration Wind
Coal
Geothermal
Petroleum Power for Biofuels, H2 Chemical(s)
transportation
Tidal
Potable
Natural Effluent Water Hydel
Reduced
Gas
effluent
Environment
CO2
capture
Fig. 19. Transition from fossil fuel based energy systems to renewable based polygeneration.
K. Jana et al. / Applied Energy 202 (2017) 88–111 107
multiple utilities makes the levelized cost of electricity lower and grid technology with the optimal power with modern equipment
efficient integration of various processes increases the system effi- like dispersed generators; dispersible loads, etc. are used to get
ciency which is both economically and environmentally good. The an optimal power flow in the smart energy systems where the
result of life cycle assessment of polygeneration shows that it is sources are different. In the power feeding to the grid, frequency
environmentally better than stand-alone units generating the matching is an important issue. Khooban et al. [213] described a
same utilities [89]. In a case study for a remote off grid Indian vil- robust adaptive control strategy to match the frequency of power
lage, it is seen that the levelized cost of electricity is decreased coming from various generators. Thus the storage plays an impor-
from 8 INR (with electricity as the only utility) to 4.2 INR when tant role in the design of the smart energy systems. Polygeneration
other utilities like ethanol and cooling are added [68]. may be an effective way to serve the purpose of both the storage
Weidou et al. depicted the need of polygeneration in the Chi- and efficient use of energy resources.
nese context. The paper emphasizes on process integration for
the efficient use of the natural resources [206]. Serra et al. 12. Conclusion
described that both the resources energy and water which are
essential for the sustenance of our civilisation needs proper With a backdrop of fast depleting fossil fuel and climate change
resource management due to the economic and the demographic due to emission of CO2, energy sector is facing the critical challenge
rise of the global population [6]. Polygeneration and process inte- of innovation of new sustainable systems. Increasing efficiency,
gration is a good means for this as it doubles the objective of effi- reducing pollution – specifically mitigating CO2 emission and opti-
cient use of natural resources and minimizes the environmental mum use of available resources are the critical challenges for
degradation effect. Hetland et al. discussed about the de carboniza- developing sustainable energy systems. Integrating multiple
tion of the energy sector in the European and Chinese conditions inputs with multiple utility outputs in a single system is called
through polygeneration by generating the multiple utilities [207]. polygeneration. With efficient integration such systems are of high
The group also suggested the carbon capture in a coal based poly- efficiency and environment friendly depending on type of fuel
generation is beneficial from environmental aspect. Bellosio et al. used. Moreover with proper matching of available resources and
described the need of process integration for the supply of energy utility demands, optimum resource management may be done,
from renewable. In the city of TORINO in the POLYCITY project of i.e., one of the key issue for sustainability.
the European Commission there is a integration of the combined In literature several theoretical description and assessment of
heat and power system coupled with an existing district heating polygeneration are available. However, prototype development
system and an absorption chillers to achieve benefits in terms of and experimental assessment of performance is very scarce. Pro-
energy efficiency [208]. Dincer and Acar described the essence of posed polygenerations using renewable are mostly of smaller
3S systems for the design of a sustainable energy system. The 3S capacity depending on available local resources and hence, dis-
signifies source, system and service. For a sustainable system, the tributed in nature. On the other hand coal based polygeneration
process integration and multi generation are emphasized. The sus- will be mostly feasible for large scale systems with added advan-
tainable systems are meant to deliver dependable, efficient, practi- tage of producing utility outputs from captured CO2. Hybrid
cal and clean power [209]. options combining both fossil and renewable inputs are also
reported in literature. As polygeneration includes multiple inputs
11. Smart energy management system with storage and outputs, optimum capacity determination based on several
technologies objectives is a critical issue. Optimization of polygeneration using
several mathematical models is reported in literatures. Perfor-
Power demand does not always conveniently match with sup- mance assessment of polygeneration is multi dimensional with dif-
ply. Hence for a reliable power supply, suitable storage systems ferent objectives. A few publications are available in this respect.
are necessary. The most conventional practice is storing the elec- Overall review on polygeneration indicates that it emerges as a
tricity in batteries. These batteries increase the cost of electricity sustainable energy solution as an efficient, environment friendly
as they require periodic replacement. Moreover, the batteries emit and optimally utilizing available natural resources.
toxic substances when they malfunction or at the time of their dis- Future research on polygeneration for successful development
posal [210]. In electricity generation system the components are may be in developing prototypes based on optimal theoretical
sized to meet the maximum demand. So there is excess electricity results and subsequent performance and feasibility assessment.
at the time when the load is less than the maximum demand. With variable inputs and outputs, intelligent monitoring and con-
There are two options to manage this. The options are (a) to store trol is critical for efficient polygeneration. Performance being multi
the electricity in a storage device to use at the time of need. (b) to dimensional, criteria of assessment of polygeneration may be sev-
use the surplus resources used in producing electricity to synthe- eral, based on objective of assessment or weighted average of sev-
size some other utilities like chemicals, bio fuels, etc. for proper eral objectives. Defining such criteria will be another interesting
resource management and (c) to sell the excess electricity to some issue for future polygeneration research. Integrating multiple util-
other areas where there is a need. The storage is still not an eco- ity outputs in efficient ways was the basic motive of developing
nomic and environmentally benign option as discussed earlier. polygeneration and this will remain for future development of
Selling of electricity is not a viable option for decentralized gener- innovative integration satisfying availability of resources and utility
ation as the load centres are dispersedly located. So in case of demands. Integrating new device/component with newer inven-
decentralized polygeneration, sometimes the electricity producing tions will always remain a scope for developing better polygenera-
resource (like syngas) is diverted to produce a bio fuel ethanol tion. Renewable inputs are generally intermittent and suitable
when the load is low [68]. In locations where there is variable time storage system integration may be another future research need.
tariff, storage may reduce the levelized cost of electricity [211]. In summary, following issues are observed through this review
Telaretti et al. compared the performance of four types of batteries of available literature on polygeneration:
namely the Li-ion battery, zinc based, advanced lead acid, zinc
based, NaS and a flow battery in places with peak demand charges Depletion of fossil fuels and climate change has forced to
and variable tariff. Their analysis reveals that zinc based, lithium develop sustainable energy solutions with higher efficiency
ion and the flow batteries give the best performance [212]. Smart and optimum resource utilization. Polygeneration emerges to
108 K. Jana et al. / Applied Energy 202 (2017) 88–111
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