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IEEE Transactions on Dielectrics and Electrical Insulation Vol. 15, No.

4; August 2008 1131

A New Dielectric Response Model for Water Tree Degraded


XLPE Insulation – Part A: Model Development
with Small Sample Verification
Andrew J. Thomas and Tapan K. Saha
University of Queensland
School of Information Technology and Electrical Engineering
Brisbane, QLD 4072, Australia

ABSTRACT
Water tree degradation in underground XLPE insulated cables is a growing, world-
wide problem. This form of degradation is ultimately fatal for affected cables, and
therefore the detection of damaging trees in power cable insulation is vital for
distribution companies to avoid catastrophic failure. Dielectric response
measurements, in both the time and frequency domains, can generate valuable
information about the condition of the cable. However, the interpretation of how these
dielectric response measurements relate to water tree density and length is a difficult
task. This paper will present a new dielectric response model for water tree degraded
XLPE insulation. The model is based on finite element analysis to determine the
electrical behaviour of water tree degraded insulation. Preliminary simulations will
verify the model development by comparing the results to small sample Pulsed Electro-
Acoustic (PEA) measurements performed by other researchers. The importance of a
strong non-linearity mechanism for accurate modelling will also be elucidated.
Index Terms — water trees, cross linked polyethylene insulation, finite element
method, dielectric measurements, space charge, conductivity, dielectric loss,
nonlinearities.

1 INTRODUCTION enhancement above the norm at the tree tip, with the general
aim of deducing the cause of water tree induced failure, which
WATER tree degradation is one of the most serious of course is an important area of study. However, a water tree
afflictions that can occur within underground medium voltage
model which is to be used in interpreting dielectric response
cross-linked polyethylene (XLPE) cables. Because of this
measurements will need to be dynamic, as dielectric response
fact, many studies have been performed concerning how water
measurements usually cover many decades of time or
trees grow, how they bring about failure and how they can be
frequency. In addition to this, the model will need to consider
detected. Perhaps the best way to fully understand the
non-linear effects with charging voltage, as this is an often
previous points is through modelling, which can analytically
observed measurement phenomena.
describe the physical situation. Water tree growth is somewhat
The authors of [3] developed a model investigating a
inevitable in XLPE cables under certain conditions. Therefore,
mechanical non-linearity mechanism, which involved the
it is a useful exercise to develop a model which can relate
opening and closing of conducting channels between voids
dielectric response measurements to the water tree degraded
under Maxwell stresses. However, this model was developed
condition of a cable, which aids in the cable diagnosis. This
to prove that the mechanical non-linearity mechanism could
will result in a more efficient and accurate diagnostic process.
be responsible for the observed non-linearity, and is therefore
A number of electrical behaviour models of water tree
only local i.e. its solution domain is of a microscopic scale
affected XLPE cables have been developed in the past. Many
around a number of voids and channels.
papers [1, 2] concentrate on power frequency (i.e.
Another series of papers considers the dynamics of water
capacitively) graded fields, with an emphasis placed on field
tree channels, where perhaps the best example is [4]. These
papers consider channel dynamics in the form of a Maxwell-
Manuscript received on 11 April 2007, in final form 23 January 2008. Wagner type equivalent circuit. The total capacitance and

1070-9878/08/$25.00 © 2008 IEEE

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1132 A. J. Thomas and T. K. Saha: A New Dielectric Response Model for Water Tree Degraded XLPE Insulation – Part A

resistance of the water treed region is calculated by allowing found to be on the order of >1 μm in diameter at the foot of
the size of the water treed region to expand and contract to a water tree, whereas the channels throughout the rest of the
simulate the filling of voids. The conduction in the region is tree are on the order of 10-100 nm in diameter [9].
modelled by a sinh dependence on the electric field, with the The interface between a water tree and XLPE within an
strength of the sinh dependence governed by a value h. The insulation can easily be considered to be a rather
authors allow the size of the water treed region and the value h complicated structure. On a macroscopic scale (on the scale
to vary (along with the low field conductivity of the region, of the water tree length itself), it is likely that there is a
which varies little) at different applied voltages in order to decay of void and channel density near the tree tip, leading
match the simulated and measured data. However, allowing h to a change in conductivity and permittivity that is not
to vary along with the size of the water treed region with instantaneous, but diffuse. There is also the question of
voltage is perhaps physically unintuitive, as it is difficult to field assisted opening and closing of water tree channels
find a physical reason as to why any change of this variable through Maxwell forces, which will be investigated further
should occur. in later sections.
Therefore in order to expand beyond the scopes or In addition to this, the electro-osmosis water tree growth
limitations of the previously mentioned papers, this paper will theory, reviewed in [11], sensibly proposes that it is likely
detail the investigation towards a new electrical model for that ionic species will diffuse, in an electrically assisted
water tree degraded XLPE. The goal of this model is to manner, into the polymer beyond the tree tip. This diffusion
macroscopically describe the electrical behaviour of water of impurities will likely increase the concentration of
trees in XLPE under certain applied electrical conditions, on hopping sites located close to the conduction band,
the scale of the water tree length itself. The overall goal of this increasing the conductivity and permittivity somewhat
study is to enable a more refined understanding of the effect of beyond the tree tip. This effect is also likely to result in a
water trees on dielectric response measurements, with the macroscopic conductivity and permittivity profile that is
actuation of this goal shown in the accompanying paper [5]. relatively gradual.
However, before such an application can be realised, an In order to model the electrical behaviour of water tree
electrical model for water tree degraded insulation must be degraded insulation, it is vital that this interfacial region is
developed and verified, which is the content of this paper. considered properly, as this region will dominate the
In Section 2, the details of a constructed one dimensional electrical characteristics of the local material. These
finite element model will be given, which describes the time- considerations will be addressed in the next section.
varying electrical behaviour of water tree degraded XLPE
insulation. Particular attention is payed to simulating the 2.2 PERMITTIVITY AND CONDUCTIVITY
space charge build up at the interface between the water tree REPRESENTATIONS
and the healthy XLPE, with this interface being modelled
diffusely in the investigation. In order to validate the model, in In this investigation, the insulation properties will be
Section 3 the results of the simulations will be compared to macroscopically considered in one-dimension only, with an
space charge measurements performed by other researchers assumption of uniformity in the remaining two dimensions.
[6] in small sample experiments. It will be seen that in order The water tree permittivity and conductivity are considered
for the model to accurately simulate the measurements, a to be uniform up to a certain point depending on the length
mechanical non-linearity mechanism based on Maxwell forces of the water tree. Beyond this region of relative uniformity,
is needed. Section 4 will contain discussion and conclusions there will be a transition from water tree electrical
of the results of this study. This paper is a major expansion properties to healthy XLPE electrical properties (i.e. a
of the preliminary/investigative work presented in [7]. substantial decrease in conductivity, and a less substantial
decrease in permittivity). In some previous water tree
modelling exercises, this change of electrical properties has
2 MODEL DESCRIPTION been considered as an ideal boundary, with an infinitely
This section will address the technical details and sharp profile. However, for reasons stated previously, this
assumptions used to generate the model of electrical ideally sharp boundary at a macroscopic level is unlikely to
behaviour of water treed insulation. exist. Experimental evidence for a more diffuse boundary
will be shown in later sections.
2.1 STRUCTURE OF WATER TREES The exact form of the interface, with regards to the
Water trees are generally considered to consist of water decreasing profile of the conductivity and permittivity is
filled micro-voids, which may or may not have practically impossible to measure directly. However
interconnecting, conducting channels. Numerous studies inferences or postulations can be made from available
[8-10] have been performed (to name only a few), using a information and these inferences can be tested through
variety of techniques such as Transmission Electron less direct means for verification. As mentioned
Microscopy (TEM) and Scanning Electron Microscopy previously, a major proposed water tree growth
(SEM), to discover this. The largest voids generally found mechanism is electro-osmosis, whereby hydrated ions
within water tree channels are on the order of 5 μm in diffuse into the insulation beyond the water tree proper
length [9]. The connecting channels between voids were with electric field assistance [11, 12]. Diffusion of

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IEEE Transactions on Dielectrics and Electrical Insulation Vol. 15, No. 4; August 2008 1133

contaminants into XLPE has been studied previously [13, the XLPE conductivity and permittivity respectively. The
14] with the contaminants in this case being sourced from ranges of these values considered in this study are [15-17]:
the semi-conductive layer. Figure 4 in [13] shows an
Conductivity
exponential-like decay in the FTIR absorbance level
Water tree: 1x10-11 – 1x10-7 S/m
(which is related to the concentration of species) of
XLPE: 1x10-18 – 1x10-16 S/m
contaminants away from the semi-conductor layer. It is a
Permittivity (relative)
reasonable assumption that the conductivity (and
Water tree: 2.3 – 5
permittivity) of an insulation are proportional to the
XLPE: 2.3
amount of contaminants it contains. In addition to this,
the authors of [14] had some success in modelling the
It should be noted that the electrical behaviour of the
space charge levels near the semi-conductive layer using
electrode/XLPE interface in this model has been neglected,
an exponential conductivity and permittivity profile.
and therefore whatever limitations on accuracy that this
It can also be noted at this point that according to the
omission may make should be considered.
electro-osmosis theory discussed in [12] a continual
The above formulations for the conductivity and
recombination and resolvation process (the resolvation
permittivity are to be considered as the low-field
owing to osmosis and perhaps dielectrophoresis) acting on
representations. As is well known, water tree degraded
diffused ion pairs mechanically fatigues the insulation
cables exhibit dielectric response non-linearity. This non-
around the ion locations. Therefore, it is also sensible to
linearity must arise in changes with the charging voltage of
propose that permanent mechanical damage of the polymer
the electrical properties of the insulation. These changes
is proportional to the ion/contaminant diffusion profile,
will be considered in the next section.
leading to the existence of proto-voids and channels in the
tree tip region, which may enable an electrical
2.3 NON-LINEAR BEHAVIOUR OF ELECTRICAL
“reconnection” process through Maxwell stresses opening
PROPERTIES
electrically conductive paths up to these areas [3]. This
will be discussed further in Section 2.3. A change of the electrical properties in water tree
While the contaminants and diffusion processes studied degraded insulation due to the electric field, at constant
in this literature is of a different form to the ionic temperature, can occur in two conceivable ways. The first
contaminants and electro-osmosis diffusion in the water way is through electronic or hopping processes due to the
tree case, an exponential change of electrical properties lowering of potential barriers between charge trapping
through space is nevertheless intuitive in light of this centres through high electric fields. The second way was
information and a reasonably well informed hypothesis. proposed in [3], and this is due to a proposed mechanical
Therefore in this study, the conductivity and permittivity of alteration of the water tree degraded material through the
the dielectric mixture will change in an exponential manner action of Maxwell forces. Both mechanisms will be
from the water tree electrical properties to the XLPE considered in this model.
electrical properties. This interfacial change will be
modelled by the sigmoid function, given by:
1
f (x ) = (1)
1 + e −αx
W
Where α is a shape parameter. In the limit of α→∞, S1
equation (1) approaches the heavy-side step function. Using
equation (1) to express the conductivity and permittivity of S2
the modelled insulation (for a vented tree) is given by:
E

σw σp Figure 1. Potential well model showing the hopping of an electron or


σ (x ) = + (2) negative ion over a potential barrier, from site S1 to S2. Arrows show both
1 + eα ( x−k ) 1 + e −α ( x − k ) a classical ‘jump’ over the potential barrier and a quantum mechanical
tunnelling through the barrier.

εp Figure 1 shows the mechanism of hopping or tunnelling


εw
ε (x ) = + (3) (electron) of a negative carrier over a potential barrier
1 + eα ( x −k ) 1 + e −α ( x − k ) lowered by an applied electric field. In solid insulation,
carriers do not move freely through the material, but rather
In equations (2) and (3), k is a location parameter ‘hop’ between localised trapping centres. In order for this
determining the spatial location in the x-direction of hop to occur, the carrier must gain thermal energy sufficient
uniform water tree electrical properties. Also in equations to overcome the barrier height between adjacent trapping
(2) and (3), σw and εw are the water tree channel centres. The energy required to traverse this barrier can be
conductivity and permittivity respectively and σp and εp are significantly reduced by an applied electric field of

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1134 A. J. Thomas and T. K. Saha: A New Dielectric Response Model for Water Tree Degraded XLPE Insulation – Part A
r
sufficient magnitude. The number of charges released from Where n is the unit normal vector. If this pressure p is
trap centres is a stochastic process based on Boltzmann’s considered to act on the many interfaces between the voids
statistics, therefore, an applied electric field increases the and XLPE, it may act to open the channels between voids,
probability of a site transition taking place and thus more allowing them to fill with liquid and become conducting.
charges are released to contribute to charge flow. Over the tree cross section, this field induced pressure and
Because conductivity is a function of the number of charge subsequent opening of channels should lead to an average
carriers, it is easily seen that the prior explained process will increase in conductivity and permittivity of the area.
increase the conductivity of the material. A derivation of field Deducing the exact relationship between the Maxwell
dependent conductivity from the jump probabilities in the forces (pressure) and the conductivity analytically (through
forward and reverse directions (with respect to field) was an additional model) is not within the scope of this study.
performed in [18], with the result being: However, some experimental results can be examined to
give an indication of the empirical form of this relationship.
⎛ 2kT ⎞ ⎛ eEa ⎞ A number of Frequency Domain Spectroscopy (FDS)
σ (E) = σ 0 ⎜ ⎟ sinh ⎜ ⎟ (4) measurements were performed on accelerated, wet aged
⎝ eEa ⎠ ⎝ 2kT ⎠ cable samples. Some of these cable samples were showing
typical LC (leakage current) responses as designated in
Where a is the distance between trap centres, e is the [19], which indicate long vented tree degradation. Figure 2
charge of the carrier in Coulombs, k is Boltzmann’s shows the loss response (imaginary part of the permittivity)
constant and T is the temperature in Kelvin. of one of these cables.
A similar line of reasoning can be made to determine the
non-linearity with respect to applied voltage for the real and
imaginary parts of the permittivity. If, under an ac applied
voltage, the carriers undergo a certain hop, or multiple hops
in the direction of the field, then a polarisation will be
created. The more carriers that undergo this process due to
field assisted de-trapping the higher the complex
permittivity will be. The derivation of the field dependent
permittivity expressions can be seen in Appendix I, and are
found as:

⎛ 2kT ⎞ ⎛ eEa ⎞
ε ' (E ) = ε LF
'
⎜ ⎟ sinh ⎜ ⎟ + ε0 (5)
⎝ eaE ⎠ ⎝ 2kT ⎠

⎛ 2kT ⎞ ⎛ eEa ⎞
ε ' ' (E ) = ε LF
''
⎜ ⎟ sinh ⎜ ⎟ (6)
⎝ eaE ⎠ ⎝ 2kT ⎠

Where the subscript LF stands for low-field, with respect Figure 2. Typical measured leakage current response at differing applied
to the permittivity. The above formulations complete the voltage levels. Uo -> rated voltage
proposed electronic or hopping non-linearity mechanism.
The second non-linear mechanism that will be These degraded samples had loss slopes inversely
considered in this work is the mechanical mechanism. This proportional to frequency, which strongly suggests that the
mechanism for non-linearity was proposed in [3]. The conduction of the samples was completely dominated by
mechanism is based upon the observed structure of water long vented trees. Therefore, assuming that the Maxwell
trees consisting of voids with interlinking channels. The forces non-linearity mechanism, as proposed in [20], is the
authors of the referenced study consider these interlinking dominant non-linearity mechanism, the square of the
channels to be closed, and therefore non-conducting under applied voltage (and therefore applied field) versus the 0.01
low-field conditions, but with an opening of these channels, Hz, low frequency loss will give the relationship between
and conduction within them, under high field conditions. the Maxwell forces and the conductivity of the long water
The explanation given as to the source of the energy tree/s. The square of the applied voltage and the low
required to open these channels is Maxwell forces due to frequency loss for the cable samples showing leakage
the electric field within the region. These Maxwell forces current behaviour were found to be exponentially related,
are a pressure acting on a 2-dimensional surface in the with the exponential fitting having R2 values in the range of
direction of the electric field, with this pressure being 0.9-0.98, therefore signifying a likely exponential
related to the electric field and permittivity as: relationship.
(
1 r r r 1
)
r Therefore, in this study, we assume the relationship of
p= E D ⋅n = ε ⋅ E2 (7)
2 2 conductivity to pressure to be:

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IEEE Transactions on Dielectrics and Electrical Insulation Vol. 15, No. 4; August 2008 1135

⎧ 2.4 TIME-VARYING FINITE ELEMENT MODEL


⎛ p⎞
⎪σ LP exp⎜ ⎟ ; σ < σ w
σ ( p) = ⎨
As mentioned previously, the Finite Element Method
⎝ A⎠ (8) (FEM) model developed in this investigation will be
⎪ σw ; σ >σw constrained to one dimension, with the assumption of

constancy in the other directions. Therefore, the form of
where the subscript LP stands for low pressure with Poisson’s equation to be solved in rectangular co-ordinates
respect to the conductivity, and A is a constant whereby to will be:
scale the strength of the effect of the pressure to
conductivity. As mentioned, the form of equation (8) is ∂ ⎛ ∂ ⎞
empirically derived from low frequency FDS data of ∇ ⋅ (− ε∇V ) = ⎜−ε V ⎟ = ρ (10)
degraded cable samples. The expected physical action of ∂x ⎝ ∂x ⎠
the equation is the mechanism as described in [3],
whereby Maxwell forces acting on the void/XLPE Where ρ is the charge density. In cylindrical co-
interfaces force open channels connecting voids, allowing ordinates, Poisson’s equation is of the form:
the region to become more conductive. In this case, it is
supposed that the “root” of the tree has permanently 1 ∂ ⎛ ∂ ⎞
connected voids and channels which lead to a uniform ⎜− ε r V ⎟ = ρ (11)
conductivity and hence the Maxwell forces will not act to
r ∂r ⎝ ∂r ⎠
increase the conductivity in this area; see equation (8). It
is postulated however that the Maxwell forces act on the Equations (10) and (11) are instantaneous in time, so in
area of damaged insulation beyond the tree or “root” tip, order to solve for the potential in a time-varying fashion,
causing channels between voids in this area to become the continuity of current equation must be applied:
conductive and leading to enhanced conductivity of the
∂ ∂ dρ
J c = (σE ) = −
area.
The permittivity in this study is postulated to be ∇J c = (12)
∂x ∂x dt
logarithmically related to the conductivity, in mechanical
non-linearity situations, as shown in equation (9). Where Jc is the conduction current density. The
Equation (9) simply expresses a linear proportionality of conduction current density can easily be obtained through
the permittivity to the logarithmic variation of the the multiplication of the space dependent conductivity and
conductivity, so that when the conductivity is changed electric field. The method for the time evolution of the
due to Maxwell forces the permittivity is also changed in space charge and subsequent potential and electrical field
a linearly proportional way to the logarithmic change in used in this investigation is the time-stepping method. The
the conductivity. This relationship is assumed due to the routine for the method is as follows:
fact that if the conductivity is increased due to Maxwell
forces to a value whereby it is equal to the assumed water 1. At time t=0, assume ρ = 0 throughout material.
tree “root” conductivity, then the permittivity in this area
should also be increased to the assumed water tree 2. Solve (10) or (11) using FEM.
permittivity. 3. Use solution in 2 to calculate differential of
conduction current density.
ε p −ε w 4. Calculate change in charge density and perform non-
ε (σ ( p )) = log(σ (x, p )) linear material calculations over time step, dt.
⎛σ p ⎞ 5. Repeat steps 2-4.
log⎜⎜ ⎟

⎝σ w ⎠
(9) Step 2 in this routine requires a solution of Poisson’s
⎛ ⎞
⎜ ⎟ equation using the Finite Element Method. The type of
⎜ ε p −ε w ⎟ FEM used in this investigation is the Garlekin method. A
+ ⎜ε p − log(σ p )⎟ comprehensive treatment of the Garlekin method, and FEM
⎜ ⎛σ p ⎞ ⎟ in general can be found in [21, 22]. Therefore, only a brief
⎜ log⎜⎜ ⎟
⎟ ⎟
⎝ ⎝σ w ⎠ ⎠ discussion on the method will follow.
The FEM consists of solving analytically unsolvable
differential equations through the use of an approximation
The effect of the constant A will be investigated in technique. This approximation technique involves breaking
following sections. Both of the non-linear electrical up the solution domain into a number of finite elements, and
property mechanisms, in analytical forms elucidated assuming the solution variable to vary polynomially between
previously, will be considered in this investigation. With element nodes (with the nodes bounding the elements).
these material properties now defined, a time-varying finite Generally the solution variable is considered to vary linearly
element model of the water tree degraded insulation can be or quadratically within the element. In this model we will
considered. consider the solution variable to vary linearly between nodes.

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1136 A. J. Thomas and T. K. Saha: A New Dielectric Response Model for Water Tree Degraded XLPE Insulation – Part A

The function that governs the variance of the solution Due to the linear nature of the interpolation functions
variable is called an interpolation function. The brief (and therefore the weighing functions in the Garlekin
mathematical treatment of the FEM is based on explanations method), equation (17) is now solvable for V through linear
given in the aforementioned references [21, 22]. algebraic methods, given appropriate boundary conditions
If the general form of the differential equation is to make the solution unique. In this investigation, the
considered, it can be represented by: boundary conditions for each solution of equations (10) or
(11) are the potentials at the electrodes.
L(φ ) − f = 0 (13) This ends a brief description of the method used to solve
for the potential, and also therefore the electric field. The
solution domain Ω, whose size is governed by the thickness
Where L is a general differential operator acting on Ф
of the insulation, is segmented into 1000 elements for this
and f is the forcing function acting on Ф (charge density in
study. The valid solution domain can be considered to exist
equation (10) or equation(11)). This approximation of the
within the proposed water tree structures, interface and
solution variable Ф (the potential V in the solution of
healthy XLPE segments in the x direction, and applicable in
Poisson’s equation) through the use of interpolation
the y and z directions where approximate uniformity holds
functions can be considered mathematically by:
in the electrical properties of the material.
∧ P
φ ( x ) = ψ ( x ) + ∑ a n Fn ( x ) (14) 3 SMALL SAMPLE INVESTIGATION
n =1 In order to access the accuracy of the model, or its ability
to reproduce physical situations faithfully, it was decided
Where P is the number of interpolation functions that the model would be tested on a small sample, space
defining the solution domain Ω, an is a constant defining charge measurement study performed in [6]. In this way,
the magnitude of the nth interpolation function, Fn is the the space charge profiles produced by the model could be
nth interpolation function and ψ is a function that satisfies compared to measurement results on a small scale
the Dirichlet or essential boundary conditions. It is now experiment, before being extended for use onto large scale
clear that the Ф representation in equation (14) is no longer cable specimen geometries.
exact for finite P, so now a residual, R, will exist in
equation (13), which is a measure of the inaccuracy of the 3.1 MEASUREMENT DETAILS
approximation, such as: This subsection will briefly address the measurement
details as given in [6]. The researchers used the Pulsed-
⎛∧⎞ Electro Acoustic (PEA) method to measure volume space
R = L⎜ φ ⎟ − f (15) charge densities within the bulk of water tree aged, small
⎝ ⎠ sample specimens. The samples measured in the
aforementioned study were 1mm thick, laboratory aged
The objective of the finite element method is to minimize specimens. An FeSO4 solution, with concentration of 0.5
this residual R. This minimization can be achieved through M/L, was applied to the sample to encourage initiation and
the use of weighing functions, w, which are multiplied growth of water trees. After 800 h of 7 kV (peak), 5 kHz
throughout equation (13) to obtain an integerable solution voltage application, water trees were found uniformly over
expression: the voltage application electrode area, with the trees being
of sufficient length to reach the centre of the sample.
⎡ ⎛ P ⎞ ⎤
∫Ω i ⎢⎣
w L (
ψ ) + L ⎜ ∑ a n Fn ⎟ − f ⎥dΩ = 0 (16)
During measurement of the space charge profile, a 7 kV
(peak) voltage was applied at varying frequencies, 50 Hz,
⎝ n =1 ⎠ ⎦ 0.1 Hz, 0.01 Hz and dc. Two dc measurements of note
were made. One of these dc measurements consisted of the
The Garlekin method involves choosing the weighing application of the dc voltage for 1 h, followed by a shorting
functions from the same set as the trial functions (while of the sample for a further hour, with space charge
keeping functions linearly independent) i.e.: measurements being made sporadically during these
intervals. The other of these dc measurements consisted of
wi ( x ) = Fi ( x ) the application of a dc voltage, followed immediately by
the space charge measurement.
In the case of solving Poisson’s equation, this gives an Seven different samples are measured in the referenced
integrand of (from (16)): study. Four of these samples are labelled A,B,C and D, and
were aged for 300, 400, 800 and 1200 h, respectively,
under the previously mentioned conditions. The other three
L ⎡d ⎛ dV ⎞ ⎤ samples W, D1 and D2 were each aged for 800 hours, but
∫0
w⎢ ⎜ − ε
⎣ dx ⎝
⎟ + ρ ⎥dx = 0
dx ⎠ ⎦
(17)
with moisture contents of 1310 (parts per million) ppm, 480
ppm and 50 ppm respectively.

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IEEE Transactions on Dielectrics and Electrical Insulation Vol. 15, No. 4; August 2008 1137

3.2 PEA MEASUREMENT DETAILS AND conductivity and permittivity between the water
IMPLICATIONS tree/XLPE interface. The resolution in this case is set to
This section will address briefly certain considerations 100 µm.
that need to be taken into account when interpreting
Pulsed-Electro Acoustic measurement results. The PEA
measurement method involves the application of short
voltage pulses to a measurement sample. These voltage
pulses exert a force on any charges within the sample,
and these charges in turn launch acoustic waves
throughout the sample to be measured by a pressure
transducer. Comprehensive descriptions of the PEA
method can be found in [23, 24].
Of particular interest in this study is the attainable
resolution of the PEA systems whose results are being
analysed in this paper. The theoretical space resolution
attainable within a PEA system is given by [23]:

Δl = vΔt (18)

Where Δl is the space resolution, v is the velocity of


propagation of the acoustic wave (approximately 2000 Figure 3. Comparison between simulated space charge profile and
m/s in polyethylene [23]) and Δt is the time-width of the resolution adjusted profile
applied voltage pulse. This finite resolution will act to
broaden in space any actual space charge profile in the
measurement results. In addition to this, attenuation and It can be observed in Figure 3 that the resolution
dispersion effects can also act to broaden the space adjustment can have a very significant effect on the charge
charge profiles, although in [25] it was found that LDPE profile; however the effect isn’t quite as significant for
(and presumably by extension XLPE) was a non- broader simulated profiles. The area under both displayed
dispersive material. In [23], PEA measurements were profiles is the same (net charge density), so it can be seen
performed on a 2 mm thick LDPE specimen, using a that the resolution simulation operation manipulates the
voltage pulse width of 30 ns. The theoretical space profile in the correct fashion. All simulated space charge
resolution, using equation (18), is therefore profiles to be compared with PEA measurements in the
approximately 60 µm. However, the authors of the study following sections will be resolution corrected.
found a resolution of 100 µm was the minimum
achievable, which is a 67% increase on the theoretical 3.3 COMPARISON OF RESULTS
resolution. This section will compare the measurements of the
The implications for this on interpreting PEA previously described experimental setup with the
measurement results is that the actual space charge simulations from the model. However, first it is pertinent to
distributions may be somewhat narrower in space than examine the experimental evidence for the hypothesis that
the measured distribution. Within the resolution range the water tree/XLPE interface is macroscopically diffuse,
however, “only the net charge density can be obtained” instead of an ideal boundary. If the interface does
[23]. Therefore, in order to effectively compare model approximate an ideal boundary, the space charge
simulations (which of course produce “actual” space distribution due to the interfacial polarization should ideally
charge distributions) with those obtained by PEA be a surface charge and approach an impulse function. A
measurements, the finite resolution must be applied to possible example of an approximation of such a distribution
the simulated results. This can be estimated by applying can be observed in Figure 3, with regards to the “actual”
a moving average filter to the simulated distribution, space charge profile. After resolution is taken into account,
with a window size equal to the resolution. This is it can be observed that the high and narrow space charge
supported by a mathematical study of the PEA density is reduced in magnitude and broadened. The spatial
measurement system performed in [26], which found that extent of the resolution corrected distribution is 100-130
the PEA signal is a weighted running average of the µm. Therefore, it can be said that any space charge
space charge distribution. distribution due to a water tree/XLPE interface that is
A demonstration of this adjustment of the simulated significantly greater than the PEA measurement system
space charge profile can be observed in Figure 3, resolution has some spatial extent. A space charge profile
whereby the model is used to produce a very localised with spatial extent at such an interface strongly suggests a
space charge profile in the same geometry and applied relatively gradual electrical properties profile if equation
voltage as that in [6], by creating a very sharp change in (12) is considered.

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1138 A. J. Thomas and T. K. Saha: A New Dielectric Response Model for Water Tree Degraded XLPE Insulation – Part A

If Figure 4 is carefully examined along with Figure 6 From the previous analysis, it is clear that the diffuse
from [6], it can be observed that the spatial extent of the water tree/XLPE interface hypothesis has been confirmed.
space charge profile due to the water tree/XLPE interface Therefore, the rest of this section will be dedicated to
is approximately 330-350 µm. The theoretical resolution comparing the model results and space charge
for the PEA measurement system used in [6] is 60 µm measurements in detail. Figures 4 and 5 show the time
(pulse width of 30 ns), so assuming that the same resolved space charge profile under ac voltage excitation
mechanisms occur as in [23], the resolution can be for sample W, and the maximum space charge density of
assumed to be equal to 100 µm. Therefore, it is clear that samples W, D1 and D2 for differing applied frequencies,
the water tree/XLPE interface in [6] cannot be considered respectively [6].
to be an ideal boundary. To give further support to this
generally, the results of a higher resolution system [27]
can be analysed.

Figure 5 Maximum space charge profiles for varying frequency applied


voltages (50 Hz, 0.1 Hz, 0.001 Hz and dc) for samples W, D1 and D2.

Figure 6 shows the model space charge density


simulation for a tree bridging half of the 1 mm thick
Figure 4 Time resolved space charge profiles under 7 kV 50 Hz ac voltage insulation, with an applied voltage of 7 kVpeak, 50 Hz at
application, sample W. the phases of 108o and 288o, which are the maximum
space charge profiles. The space charge profiles are
The resolution given in [27] is 10 µm, however this resolution corrected, and the water tree conductivity is
corresponds to the theoretical resolution of the PEA equal to 5x10-8 S/m.
system using equation (18) (pulse width of 5 ns). By examining Figure 6, it can be observed that the
Therefore, in order to be conservative, 40 µm is added to simulated space charge density corresponds very well to
give an assumed resolution of 50 µm (in [23], the actual the space charge density as shown in Figure 4, at its
resolution is 40 µm greater than the theoretical maximum values of 108 and 288 degrees. It can be
resolution). The sample to be analysed in [27] is a 0.5 mm observed in Figure 4 that the spatial extent of the space
thick XLPE specimen, with water trees grown to the charge density is approximately 350 µm, with a maximum
centre of the sample. If Figure 5 (a) in [27] is carefully space charge density of 1.6 C/m3. The maximum space
examined, it can be observed that the space charge profile charge density follows the applied voltage with a slight
due to the water tree/XLPE interface has a spatial extent lag, as in Figure 5, with the maximums occurring at 108
of approximately 170 µm. This again supports the and 288 degrees. Figure 7 shows the total charge versus
hypothesis that the water tree/XLPE interface is gradual the applied voltage, with the total charge being calculated
in its electrical properties. The two examples given by integrating the charge density in Figure 6 and
previously are for samples with likely numerous trees multiplying it by the electrode area given in [6]. It can be
uniformly reaching the centre of the samples, however the observed that the total charge behaves linearly with
same diffuse interface can be observed for single trees, applied voltage, and is practically identical to (A-1),
see Figure 4 in [28]. Figure 5 in [6].

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IEEE Transactions on Dielectrics and Electrical Insulation Vol. 15, No. 4; August 2008 1139

It can be observed that the simulated space charge profiles


in Figure 9 match well with the measurements shown in
Figure 8. The conductivity of the water treed region in Figure
9 is 5x10-11 S/m, which is within the range of reported
conductivities in the literature. As can be observed, the water
tree conductivity used in Figure 9 is much below that of
Figure 6. This reduction is supported by the results shown in
Figure 5. It can be observed in Figure 5 that the samples that
were dried (D1 and D2) have a reduced maximum space
charge magnitude (compared to sample W), and that this
magnitude takes considerably longer to saturate (if it does at
all within the applied voltage time frame, this is hard to tell
visually) under dc voltage conditions.

Figure 6. Simulated space charge density for a water tree bridging half the
insulation thickness, at phases of 108o and 288o.

Figure 7. Total integrated charge at 108 degrees versus applied voltage


Figure 8. 7 kV dc space charge measurement on four aged samples, A, B,
The nature of the space charge build up at the interface of C and D [6].
the water tree and XLPE is due to interfacial polarisation, as
argued for convincingly in [6]. This interfacial polarisation is
due mainly to the large decrease in conductivity at the water
tree/XLPE interface. As the relatively large conductivity of
the water tree is likely due to the presence of ionic carriers
[16], the space charge distribution at the tree tip is almost
certainly comprised of ions. It is also possible that beyond
the tree tip, due to the electro-osmosis hypothesis of water
tree growth, the diffusion of ionic impurities and therefore
the likely existence of impurity states relatively close to the
conduction band, that ionic hopping between traps/impurity
sites occurs.
The dc behavior of the water trees can also be
examined with the model. Figure 8 shows the space
charge measurements for samples A, B, C and D in [6] Figure 9. Simulated space charge profiles for 7 kV dc voltage application
under 7 kV dc voltage application. The measurements (one second after voltage application) with 4 different water tree lengths.
were made “immediately after the dc voltage application”
[6]. By examining Figure 7 in [6], it can be observed that If the space charge process is considered via a simple
trees bridging increasingly greater percentages of the Maxwell-Wagner interfacial model, the time constant for
thickness of the insulation moving from sample A to D. the build up of the interfacial space charge can be
Figure 9 shows the simulated space charge density after 1 determined essentially by the ratio of the dual permittivity
s of voltage application (in an attempt to replicate the and the water tree conductivity (XLPE conductivity can be
measurement being made “immediately” after the dc neglected in this simple model due to its small magnitude).
voltage application). If the charge build up process can be roughly approximated

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1140 A. J. Thomas and T. K. Saha: A New Dielectric Response Model for Water Tree Degraded XLPE Insulation – Part A

by this mechanism, than a slower build up of charge (longer


time constant) can be explained through a reduced water
tree conductivity. Because the magnitude of maximum
space charge density in Figure 8 is equal to approximately 1
C/m3, which is somewhat close to the magnitude of samples
D1 and D2 in Figure 5 (which almost certainly have a
reduced water tree conductivity due to drying), a lower
conductivity for the simulation of Figure 8 was deemed
necessary. According to the model results, which clearly
can reproduce the profiles of Figure 8 accurately, it is
unlikely that the space charge profiles of Figure 8 have
reached a steady state value.
The previous discussion is an effective segue to the
discussion of the clear steady state behaviour of sample
W under dc voltage application as shown in Figure 5. For
Figure 10. Simulated space charge profiles for 7 kV dc voltage
sample W, within 60 s the maximum space charge density application, non-linearity mechanism omitted.
has reached its highest value, approximately 1.5 C/m3. It
was found that, in replicating this saturation of the
maximum space charge density with the model that the This redistribution of electric field is performed by a
Maxwell forces based non-linearity mechanism plays an redistribution, or general build up, of charge. This build up
important part. When no non-linear mechanisms are being of charge takes time, depending on the time constant of the
considered, the only explanation for a steady state space dielectric region, therefore giving a different charge
charge density for sample W is a close to ideal boundary distribution at different times as seen in Figure 10. By
between the water tree and XLPE interface. Because of including equation (12) in Poisson’s equation (10), the
the very slow time constant of such an interface, the following expression can be derived (see Appendix II):
movement of charge into a close to ideal boundary is
r ⎛ ε ⎞ ε ∂ρ
likely to be beyond any practical measurement time. ρ = J ⋅ grad ⎜ ⎟ − (19)
However, as was discussed previously, the measured ⎝ σ ⎠ σ ∂t
space charge profiles in the literature, and the successful
simulations shown in this section, strongly suggest a It can be seen in equation (19) that at steady-state (with
diffuse boundary, with a relatively gradual change of regards to charge density), the static charge density will
electrical properties. The simulation results of a diffuse depend on the spatially uniform current density and the
interface, with electrical properties the same as that which spatial gradient of the ratio of the permittivity to the
produced Figure 6, without the inclusion of a non-linear conductivity. Therefore, after a steady state develops, at
mechanism, under 7 kV dc voltage application can be any gradient of the ratio of the permittivity to the
observed in Figure 10. conductivity will yield a time-independent charge density.
By examining Figure 10, it can be observed that the In order to cease this movement of charge through the
space charge profile, while initially resembling those in interface, and therefore cease its build up in magnitude so
Figure 4 at short times, continues to grow in magnitude and that it reaches a steady state on the order of 1.5 C/m3 as in
shift to the right (towards to the negative electrode). It is Figure 5, it is required that there is a negligible gradient
clear that this behaviour of the space charge is in gross of the ratio of the permittivity to the conductivity beyond
contradiction with the dc space charge behaviour of sample the observed charge magnitude in the centre of the
W, shown in Figure 5. This behaviour can be understood in sample.
two ways. First, the build up in magnitude of the total The introduction of the mechanical non-linearity
charge (positive and negative) can be explained through the mechanism solves this problem. Figure 11 shows the
simple, parallel plate, charge-capacitance relationship. As evolution of the space charge density in the sample when
the distance between the ‘plates’ (in this case, the distance the mechanical non-linearity mechanism is enabled, with an
between the active space charge region and the opposing A value of 350 Pa in equation (8). It should be noted that all
electrode) decreases, in order to keep the voltage constant, simulations shown previously, apart from Figure 10, have
the total charge on the ‘plates’ must increase. had the non-linear mechanism enabled with an A value of
The shift to the right over time of the charge grouping, 350 Pa. Figure 12 shows the corresponding simulated
can be explained through an analysis of Poisson’s and the change in the conductivity profile over time.
continuity equation. By examining equation (12) it can be A steady-state condition in terms of the space charge
seen that for a steady state charge density to prevail in a profile is achieved after approximately 50 ms. This result
conductively inhomogeneous medium, the electric field can be compared to that seen in Figure 10, whereby the
must redistribute in such a way as to cancel the rate of steady state condition has not developed after 5 s and with a
change, in space, of the conductivity. space charge magnitude in gross contradiction with the

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IEEE Transactions on Dielectrics and Electrical Insulation Vol. 15, No. 4; August 2008 1141

results seen in Figure 5. The behaviour seen in Figure 11 is mechanism, the steady state maximum charge density under
emergent after the introduction of a mechanical non- dc voltage application for sample W in Figure 5 was
linearity mechanism. This mechanism acts to flatten the impossible to replicate. This and the successfulness of the
conductivity (and therefore permittivity) profile in the non-linear enabled model in reproducing the measured space
region beyond the space charge peak, as can be observed in charge profiles in Figures 6 and 9 give confidence to the
Figure 12. It can be observed that the maximum space postulated mechanism. In addition to this, the accompanying
charge in Figure 11 reaches a steady state value on the paper [5] extends this model and enables it to predict the
order of 1.5 C/m3, which agrees with the maximum dc dielectric response of water tree degraded XLPE cables. In
space charge values shown in Figure 5 for sample W. that paper, it is shown that the model can accurately
reproduce the non-linear behaviour of degraded cable
samples measured using Frequency Domain Spectroscopy.

4 DISCUSSION AND CONCLUSION


A point of note can be made at this point about the
previous simulations and the mechanical non-linearity
mechanism. As was stated previously, it was found through
extensive simulations that without the proposed
mathematical form of the mechanical non-linearity
mechanism, a steady state maximum space charge density
as displayed for sample W in Figure 5 was not possible to
obtain. Therefore, the preceding results give supporting
evidence to the general, non-analytical, mechanical non-
linearity mechanism as proposed in [3]. The electrical
Figure 11. Space charge evolution in small sample simulation, with a tree
bridging roughly 50% of the insulation.
mechanism of non-linearity described by equations (5) and
(6) was also considered. Without the mechanical non-
linearity mechanism, it was found that the electrical
mechanism caused some very slight increases in
conductivity and permittivity. However, when coupled with
the proposed mechanical non-linearity mechanism, the
effects of the electrical mechanism was negligible.
A further point to be made is regarding the acceptable
range of the mechanical non-linearity ‘turn on’ constant A.
This constant was varied through various values, however it
was found that only within the range of 300-500 Pa was a
steady state maximum space charge density attainable that
still allowed a good comparison between the space charge
profile simulations and Figures 4 and 8. In order to be
conservative with the magnitude of the mechanical non-
linearity mechanism, the highest value in this range, 500 Pa,
Figure 12. Simulated conductivity profile evolution over time under the has been chosen to be used in the second part of this study
action of the proposed mechanical non-linearity mechanism. [5]. The relatively low value of this constant may bring into
question the physicality of the model. However, it should be
The enhanced, or non-zero, space charge profile beyond
noted that this is a macroscopic simulation, and that stresses
the space charge peak in Figure 11, towards the negative
due to microscopic features such as geometrically “sharp”
electrode, is due to the proposed mechanical non-linearity
voids, may act to enhance these pressures.
mechanism resulting in a slight slope of the conductivity in
the x~0.6-0.9x10-3 region, instead of a completely flat In conclusion, this paper has detailed the development of a
response. Unfortunately, the static dc space charge dynamic electrical finite element model for water tree
distribution due to water tree degradation which has been degraded insulation. The model uses a diffuse boundary
simulated in Figure 11 has not been displayed in [6] or between the water tree and XLPE, along with an analytical
elsewhere in the available literature to the authors’ mechanical non-linearity mechanism based on the developed
knowledge. It has already been discussed that the dc space Maxwell forces within the material. By doing this, the
charge distributions shown in Figure 8 are unlikely to be simulated results incorporating the mechanical non-linearity
static distributions, being measured immediately after the dc mechanism can attain a close match to the small sample PEA
voltage application and having the characteristics of a low measurements performed in [6], without the need for any
water tree conductivity. Therefore, the non-linearity applied physical variables which change with applied
mechanism which results in Figure 11 is difficult to confirm voltage. Due to the success of the model, a second half of the
directly. However, it was found that without such a study was undertaken to extend the model in a practical role

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1142 A. J. Thomas and T. K. Saha: A New Dielectric Response Model for Water Tree Degraded XLPE Insulation – Part A

of interpreting diagnostic response measurements. This work If the real part of the permittivity is converted to
is presented in the accompanying paper [5]. susceptibility:

APPENDIX I ε'
χ = −1
'
(26)
Polarisation can be expressed both macroscopically and ε0
microscopically:
The constancy between the real and imaginary parts of
P = (ε ' − ε 0 ) E = uμ (20) the susceptibility, through the Universal Relaxation Law
[29], can be evoked to give equation (6).
Where u is the number of dipoles operating at field E and
μ is the average dipole moment. If the simplistic 2-
dimensional potential well case is considered, as illustrated APPENDIX II
in Figure 1, then the average dipole moment from the Poisson’s equation can be expressed as:
hopping of carriers can be expressed as: r r
ρ = ∇D = ∇εE (27)
N
⎛ eEa ⎞
∑ qi d i
f ( f − f ) ea
ea sinh⎜
⎝ 2kT ⎠
⎟ The conductive current density can be defined as:
μ = i =1
e f r
= = (21) r
u f e ( f f + f r )ea ⎛ eEa ⎞ J = σE (28)
cosh⎜ ⎟
⎝ 2kT ⎠
Therefore, equation (28) can be re-expressed as:
Where ff is the probability of a hop in the direction of
ε r
the field for an negatively charged carrier, given ρ =∇ J (29)
thermal emission of a carrier, fr is the probability of an σ
hop in the opposite direction, given thermal emission of
a carrier, fe is the probability of therm-e of the carrier Using the identity:

( )
r r
∇( f ⋅ A) = f ∇ ⋅ A + (∇f ) ⋅ A
and d is the distance between the dipolar charges. As
can be seen from equation (21), the simplification has
been made that all potential wells are a distance a apart
(hence d = a), and all the carriers are single charged Equation (29) can be re-expressed as:
(hence q = e). From equations (20) and (21) then, the ε r ⎛ ε ⎞ r
polarisation for the orientation processes described ρ= ∇ ⋅ J + ⎜∇ ⎟⋅ J (30)
above is: σ ⎝ σ ⎠
⎛ −W ⎞ Substituting the continuity equation (12) into equation
N exp⎜ ⎟ea (30) gives equation (19).
⎟ = (ε − ε 0 )E (22)
⎝ kT ⎠ ⎛ eEa ⎞
P= sinh ⎜ '

2 ⎝ 2kT ⎠ ACKNOWLEDGEMENTS
The authors would like to acknowledge Ergon Energy
Where N is the total number of possible dipoles in a dielectric
and the Australia Research Council for the funding that
(N is independent of E, whereas u is dependent). Rearranging
made this study possible. The authors would also like to
(22), an expression for the permittivity can be obtained:
acknowledge the project members from the Queensland
⎛ −W ⎞ ⎛ eEa ⎞ University of Technology (QUT) for their support. In
N exp⎜ ⎟ea sinh ⎜ ⎟ particular, the authors would like to acknowledge Frith
⎝ kT ⎠ ⎝ 2kT ⎠
ε (E ) =
'
+ ε0 (23) Foottit, of QUT, for the development and continual
2E maintenance of the accelerated ageing experiment, Bolarin
Oyegoke, of QUT, for his experimental advice and support
Equation (23) can be expressed without the N term by and Prasanna Wickramasuriya, of Ergon Energy, for his
using the low field permittivity: support during the measurements.
⎛ 2kT ⎞ ⎛ eEa ⎞
ε ' (E ) = ε LF
'
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Vol. 18, pp. 565-585, 1983. Information Technology and Electrical
[13] J. Bezille, H. Janah, J. Chan, and M. D. Hartley, "Influence of Engineering. He graduated from the Queensland
diffusion on some electrical properties of synthetic cables", IEEE University of Technology in 2003 with honors and
Conf. Electrical Insulation and Dielectric Phenomena, Victoria, worked in Connell Wagner’s power systems group
Canada, pp. 367-372, 1992. for one year. During that year, 10 months were
[14] J. Hjerrild, J. Holboll, M. Henriksen and S. Boggs, "Effect of spent at Connell Wagner’s Advanced Technology
semicon-dielectric interface on conductivity and electric field Centre in Newcastle, Australia within the high
distribution", IEEE Trans. Dielectr. Electr. Insul., Vol. 9, pp. 596- voltage testing division. His current research
603, 2002. interests include insulation condition assessment
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and permittivity of water tree in polyethylene", IEEE Conf. Electr. cables.
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Intern. Conf. on Properties and Application of Dielectric Materials, Bangladesh and immigrated to Australia in 1989. Dr.
Xi'an, China, pp. 455-458, 2000. Saha is a Professor of Electrical Engineering in the
[17] G. Katsuta, A. Toya, L. Ying, M. Okashita, F. Aida, Y. Ebinuma, and school of Information Technology and Electrical
Y. Ohki, "Experimental investigation on the cause of harmfulness of Engineering, University of Queensland, Australia.
the blue water tree to XLPE cable insulation", IEEE Trans. Dielectr. Before joining the University of Queensland in 1996,
Electr. Insul., Vol. 6, pp. 887-891, 1999. he taught at the Bangladesh University of
[18] J. J. O'Dwyer, The Theory of Electrical Conduction and Breakdown Engineering and Technology, Dhaka, Bangladesh for
in Solid Dielectrics. Oxford: Clarendon Press, 1973. three and half years and then at James Cook
[19] P. Werelius, P. Tharning, R. Eriksson, B. Holmgren, and U. Gafvert, University, Townsville, Australia for two and half
"Dielectric spectroscopy for diagnosis of water tree deterioration in years. He is a Fellow of the Institution of Engineers,
XLPE cables", IEEE Trans. Dielectr. Electr. Insul., Vol. 8, pp. 27-42, Australia. His research interests include power systems, power quality and
2001. condition monitoring of electrical plants.
[20] S. Hvidsten, E. Ildstad, B. Holmgren, and P. Werelius, "Correlation
between AC breakdown strength and low frequency dielectric loss of
water tree aged XLPE cables", IEEE Trans. Power Delivery, Vol. 13,
pp. 40-45, 1998.

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